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Received December 18, 2010
Accepted February 15, 2011
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Adsorption characteristics of methylene blue onto the N-succinyl-chitosan-gpolyacrylamide/attapulgite composite
College of Material Science and Art Design, Inner Mongolia Agricultural University, Hohhot 010018, P. R. China 1Center of Eco-material and Green Chemistry, Lanzhou Institute of Chemical Physics, Chinese Academy of Sciences, Lanzhou 730000, P. R. China
wl2083663@126.com
Korean Journal of Chemical Engineering, August 2011, 28(8), 1658-1664(7), 10.1007/s11814-011-0037-1
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Abstract
N-succinyl-chitosan-g-polyacrylamide/attapulgite (NSC-g-PAM/APT) composite was applied as adsorbent for the removal of methylene blue (MB) from aqueous solution. The initial pH value of the dye solutions, the contact temperature, the contact time and the concentration of the dye solutions on adsorption capacity of the composite for MB dye were investigated. The adsorption kinetics and isotherms were also studied. It was shown that all the sorption processes were better fitted by pseudo-second-order equation and the Langmuir equation. The results indicated that the adsorption capacity of the composite was higher than those of chitosan (CTS) and attapulgite (APT). The desorption studies revealed that the composite provided the potential for regeneration and reuse after MB dye adsorption, which implied that the composite could be used as quite effective adsorbent for the removal of MB from aqueous solution.
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Ngah WSW, Liang KH, Ind. Eng. Chem. Res., 38(4), 1411 (1999)
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Mckay G, Geundi MEI, Nassar MM, Process Saf. Environ., 74, 277 (1996)
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Tan IAW, Ahmad AL, Hameed BH, J. Hazard. Mater., 154(1-3), 337 (2008)
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Wong YC, Szeto YS, Cheung WH, McKay G, Adsorption., 14, 11 (2008)
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Knorr D, J. Food Sci., 48, 36 (1983)
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Juang RS, Tseng RL, Wu FC, Lee SH, J. Chem. Technol. Biotechnol., 70(4), 391 (1997)
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Sashiwa H, Shigemasa Y, Carbohydr. Polym., 39, 127 (1999)
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Sridhari TR, Dutta PK, Indian J. Chem. Technol., 7, 198 (2000)
Heras A, Rodriguez NM, Ramos VM, Agullo E, Carbohydr. Polym., 44, 1 (2001)
Wang W, Chen H, Wang A, Sep. Purif. Technol., 55(2), 157 (2007)
Chen H, Zhao J, Adsorption., 15, 381 (2009)
Zhang JP, Chen H, Li P, Wang AQ, Macromol. Mater. Eng., 291, 1529 (2006)
Zhang JP, Li A, Wang AQ, Carbohydr. Polym., 65, 150 (2006)
Paulino AT, Guilherme MR, Reis AV, Campese GM, Muniz EC, Nozaki J, J. Colloid Interface Sci., 301(1), 55 (2006)
Wang L, Zhang JP, Wang AQ, Colloids Surf. A: Physicochem. Eng. Aspects., 32, 47 (2008)
Li P, Zhang JP, Wang AQ, Macromol. Mater. Eng., 292, 962 (2007)
Bhattacharyya KG, Sarma A, Dyes Pigm., 57, 211 (2003)
Lagergren S, Kungl. Sven. Veten. Akad. Handl., 24, 1 (1898)
Mall ID, Srivastava VC, Kumar GVA, Mishra IM, Colloids Surf. A: Physicochem. Eng. Aspects., 278, 175 (2006)
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Nasuha N, Hameed BH, Chem. Eng. J., 166, 783 (2011)
Hamdaoui O, J. Hazard. Mater., 135(1-3), 264 (2006)
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Gurses A, Dogar C, Yalcin M, Acikyildiz M, Bayrak R, Karaca S, J. Hazard. Mater., 131(1-3), 217 (2006)
Kavitha D, Namasivayam C, Bioresour. Technol., 98(1), 14 (2007)
Sheng JW, Xie YN, Zhou Y, Appl. Clay Sci., 46, 422 (2009)
