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Received October 22, 2010
Accepted May 23, 2011
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Investigation of CO2 adsorption by bagasse-based activated carbon
Anusorn Boonpoke
Siriluk Chiarakorn1
Navadol Laosiripojana
Sirintornthep Towprayoon
Amnat Chidthaisong†
The Joint Graduate School of Energy and Environment, King Mongkut, Bangkok 10400, Thailand 1Division of Environmental Technology, School of Energy, Environment and Materials, King Mongkut, Bangkok 10400, Thailand
amnat_c@jgsee.kmutt.ac.th
Korean Journal of Chemical Engineering, January 2012, 29(1), 89-94(6), 10.1007/s11814-011-0143-0
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Abstract
Bagasse-based activated carbon (BAC) and amine-modified BAC were prepared and investigated for CO2 adsorption capacity. Modifying BAC with amines resulted in a decrease of surface area, but the decreasing magnitude varied depending on type and loading rate of amines. At room temperature, the unmodified BAC was able to adsorb more CO2 than the amine-modified BAC. This ability was related to the higher surface area of unmodified than that of the modified BAC. When temperature increased, CO2 adsorption capacity of all absorbents was decreased. However, above 323 K and a concentration of CO2 lower than 30% v/v, the BAC modified with PEI at 5 and 25 wt% showed higher adsorption capacity. Among all adsorbents under 15% CO2 and 348 K, BAC-PEI25 showed the highest adsorption capacity (0.20 mmol/g).
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Van Der Vaart R, Huiskes C, Bosch H, Reith T, Adsorption., 6, 311 (2000)
Maroto-Valer MM, Tang Z, Zhang YZ, Fuel Process. Technol., 86(14-15), 1487 (2005)
Pevida C, Plaza MG, Arias B, Fermoso J, Rubiera F, Pis JJ, Appl. Surf. Sci., 254(22), 7165 (2008)
Zhu T, Yang S, Choi DK, Row KH, Korean J. Chem. Eng., 27(6), 1910 (2010)
Tsai WT, Chang CY, Lee SL, Bioresour. Technol., 64(3), 211 (1998)
Onal Y, Akmil-Basar C, Sarici-Ozdemir C, Erdogan S, J. Hazard. Mater., 142(1-2), 138 (2007)
Stubington JF, Aiman S, Energy Fuels, 8(1), 194 (1994)
Ioannidou O, Zabaniotou A, Renew. Sust. Energy Rev., 11, 1966 (2007)
Sing KSW, Everett DH, Haul RAW, Moscou L, Pierott RAi, Rouquerol J, Siemieniewska T, Pure. Appl. Chem., 57, 603 (1985)
Gray ML, Champagne KJ, Fauth D, Baltrus JP, Pennline H, Int. J. Green Gas Con., 2, 3 (2008)
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