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Received November 12, 2013
Accepted January 12, 2014
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This is an Open-Access article distributed under the terms of the Creative Commons Attribution Non-Commercial License (http://creativecommons.org/licenses/bync/3.0) which permits
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Preparation, characterization and performance of cellulose acetate ultrafiltration membranes modified by charged surface modifying macromolecule
Polymeric Materials Research Lab., PG & Research Department of Chemistry, Alagappa Government Arts College, Karaikudi - 630 003, India
Korean Journal of Chemical Engineering, June 2014, 31(6), 1057-1064(8), 10.1007/s11814-014-0018-2
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Abstract
A charged surface modifying macromolecule (cSMM) was synthesized, characterized by FT-IR spectroscopy and blended into the casting solution of cellulose acetate (CA) to prepare surface modified UF membranes by phase inversion technique. With an increasing cSMM additive content from 1 to 4 wt%, pure water flux (PWF) and water content (WC) were increases whereas the hydraulic resistance decreases. Surface characteristic study reveals that the surface hydrophilicity increased in cSMM modified CA membranes. The pore size and surface porosity of the 4 wt% cSMM blend CA membranes increases to 41.26 A and 0.015%, respectively. Similarly, the molecular weight cut-off (MWCO) of the membranes ranged from 20 to 45 kDa, depending on the various compositions of the prepared membranes. Lower flux decline rate (47.2%) and higher flux recovery ratio (FRR) (89.0%), exhibited by 4 wt% cSMM blend membranes demonstrated its fouling resistant characteristic compared to pristine CA membrane.
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Sivakumar M, Mohan DR, Rangarajan R, J. Membr. Sci., 268(2), 208 (2006)
Ma YX, Shi FM, Ma J, Wu MN, Zhang J, Gao CJ, Desalination, 272(1-3), 51 (2011)
Kim Y, Rana D, Matsuura T, Chung WJ, J. Membr. Sci., 338(1-2), 84 (2009)
Nagendran A, Mohan D, J. Appl. Polym. Sci., 110(4), 2047 (2008)
Nagendran A, Vijayalakshmi A, Arockiasamy DL, Shobana KH, Mohan D, J. Hazard. Mater., 155(3), 477 (2008)
Rana D, Matsuura T, Chem. Rev., 110(4), 2448 (2010)
Taurozzi JS, Crock CA, Tarabara VV, Desalination, 269(1-3), 111 (2011)
Azoug C, Sadaoui Z, Charbit F, Charbit G, Can. J. Chem. Eng., 75, 74 (1997)
Lin CF, Wu CH, Lai HT, Sep. Purif. Technol., 60(3), 292 (2008)
Yuan W, Zydney AL, J. Membr. Sci., 157(1), 1 (1999)
Jung CW, Kang LS, Korean J. Chem. Eng., 20(5), 855 (2003)
Kuttowy O, Sourirajan S, J. Appl. Polym. Sci., 19, 1449 (1975)
Haddad R, Ferjani E, Roudesli MS, Deratani A, Desalination, 167(1-3), 403 (2004)
Maheswari P, Mohan D, High Perform. Polym., 25, 641 (2013)
Yeo HT, Lee ST, Han MJ, J. Chem. Eng. Japan, 33, 180 (2003)
Mosqueda-Jimenez DB, Narbaitz RM, Matsuura T, Chowdhury G, Pleizier G, Santerre JP, J. Membr. Sci., 231(1-2), 209 (2004)
Nagendran A, Mohan D, Polym. Adv. Technol., 19, 24 (2008)
Idris A, Zain NM, Noordin MY, Desalination, 207(1-3), 324 (2007)
Ochoa NA, Masuelli M, Marchese J, J. Membr. Sci., 278(1-2), 457 (2006)
Reddy AVR, Mohan DJ, Buch PR, Joshi SV, Ghosh PK, Int. J. Nucl. Desalination, 2, 103 (2006)
Cho DL, Kim SH, Huh YI, Kim D, Cho SY, Kim BH, Macromol. Res., 12(6), 553 (2004)
Suk DE, Chowdhury G, Matsuura T, Narbaitz RM, Santerre P, Pleizier G, Deslandes Y, Macromolecules, 35(8), 3017 (2002)
Rana D, Matsuura T, Narbaitz RM, Feng C, J. Membr. Sci., 249(1-2), 103 (2005)
Rana D, Scheier B, Narbaitz RM, Matsuura T, Tabe S, Jasim SY, Khulbe KC, J. Membr. Sci., 409-410, 346 (2012)
Rana D, Kim Y, Matsuura T, Arafat HA, J. Membr. Sci., 367(1-2), 110 (2011)
Suk DE, Matsuura T, Park HB, Lee YM, J. Membr. Sci., 277(1-2), 177 (2006)
Rana D, Matsuura T, Narbaitz RM, J. Membr. Sci., 282(1-2), 205 (2006)
Fang Y, Pham VA, Matsuura T, Santerre JP, Narbaitz RM, J. Appl. Polym. Sci., 54(12), 1937 (1994)
Kim Y, Rana D, Matsuura T, Chung WJ, Chem. Commun., 48, 693 (2012)
Mohd Norddin MNA, Rana D, Ismail AF, Matsuura T, Sudirman R, Jaafar J, J. Ind. Eng. Chem., 18(6), 2016 (2012)
Hamza A, Pham VA, Matsuura T, Santerre JP, J. Membr. Sci., 131(1-2), 217 (1997)
Bolong N, Ismail AF, Salim MR, Rana D, Matsuura T, Tabe-Mohammadi A, Sep. Purif. Technol., 73(2), 92 (2010)
Norddin MNAM, Ismail AF, Rana D, Matsuura T, Mustafa A, Tabe-Mohammadi A, J. Membr. Sci., 323(2), 404 (2008)
Machado PST, Habert AC, Borges CP, J. Membr. Sci., 155(2), 171 (1999)
Barth C, Goncalves MC, Pires ATN, Roeder J, Wolf BA, J. Membr. Sci., 169(2), 287 (2000)
Arthanareeswaran G, Srinivasan K, Mahendran R, Mohan D, Rajendran M, Mohan V, Eur. Polym. J., 4, 751 (2004)
Bhattacharya D, McCarthy JM, Grieves RB, AIChE J., 20, 1206 (1974)
Tamura M, Uragami T, Sugihara M, Polymer, 22, 829 (1981)
Mahendran R, Malaisamy R, Mohan D, Polym. Adv. Technol., 15, 149 (2004)
Sivakumar M, Malaisamy R, Sajitha CJ, Mohan D, Mohan V, Rangarajan R, J. Membr. Sci., 169(2), 215 (2000)
Nunes SP, Peinemann KV, J. Membr. Sci., 73, 25 (1992)
Sarbolouki MN, Sep. Sci. Technol., 17, 381 (1982)
Velicangil O, Howell JA, J. Phys. Chem., 84, 2991 (1980)
Wang YQ, Su YL, Ma XL, Sun Q, Jiang ZY, J. Membr. Sci., 283(1-2), 440 (2006)
Jayalakshmi A, Rajesh S, Mohan D, Appl. Surf. Sci., 258(24), 9770 (2012)
Baker RW, Membrane technology and applications, Wiley, Chichester, UK (2004)
Gekas V, Desalination, 68, 77 (1988)
Brinkert L, Abidine N, Aptel P, J. Membr. Sci., 77, 123 (1993)
Brousse CL, Chapurlat R, Quentin JP, Desalination, 18, 137 (1976)
Arthanareeswaran G, Latha CS, Mohan D, Raajenthiren M, Srinivasan K, Sep. Sci. Technol., 41(13), 2895 (2006)
Ousman M, Bennasar M, J. Membr. Sci., 105(1-2), 1 (1995)
Michaels AS, Nelsen L, Porter MC, Ultrafiltration in membrane processes in industry and biomedicine, Plenum Press, New York (1971)
Nakao S, Osada H, Kurata H, Tsuru T, Kimura S, Desalination, 70, 191 (1988)
Mohd Norddin MNA, Ismail AF, Matsuura T, Rana D, J. Teknol., 49, 91 (2008)
Sivakumar M, Mohan DR, Rangarajan R, J. Membr. Sci., 268(2), 208 (2006)
Ma YX, Shi FM, Ma J, Wu MN, Zhang J, Gao CJ, Desalination, 272(1-3), 51 (2011)
Kim Y, Rana D, Matsuura T, Chung WJ, J. Membr. Sci., 338(1-2), 84 (2009)
Nagendran A, Mohan D, J. Appl. Polym. Sci., 110(4), 2047 (2008)
Nagendran A, Vijayalakshmi A, Arockiasamy DL, Shobana KH, Mohan D, J. Hazard. Mater., 155(3), 477 (2008)
Rana D, Matsuura T, Chem. Rev., 110(4), 2448 (2010)
Taurozzi JS, Crock CA, Tarabara VV, Desalination, 269(1-3), 111 (2011)
