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Received February 26, 2014
Accepted April 16, 2014
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This is an Open-Access article distributed under the terms of the Creative Commons Attribution Non-Commercial License (http://creativecommons.org/licenses/bync/3.0) which permits
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Semi-empirical modeling of carbonator with the physico-chemical characteristics of sorbent activity parameterized by the partial least squares method
1Department of Chemical and Biomolecular Engineering, Seoul National University of Science and Technology, Seoul 137-743, Korea 2Department of Energy Systems Research, Ajou University, Suwon 443-749, Korea 3Department of Chemical Engineering, Ajou University, Suwon 443-749, Korea
mjpark@ajou.ac.kr
Korean Journal of Chemical Engineering, September 2014, 31(9), 1532-1538(7), 10.1007/s11814-014-0114-3
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Abstract
We developed an evaluation module to calculate the carbon capture efficiency of a fluidized bed carbonator via the semi-empirical modeling of the solvent activity of lime particles. Since the solvent activity is affected by regeneration cycle number, reactor temperature, and particle size, two design parameters for the particle activity model, i.e., the characteristic time (t*) and the maximum conversion of particles (XN), were determined as functions of the carbonator operating conditions by applying the partial least square (PLS) method to experimental data reported in_x000D_
the literature. The validity of the proposed approach was shown, and the effects of reactor design factors on the carbonator performance are discussed by means of appropriate simulation studies.
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Park MJ, Dokucu MT, Doyle FJ, Ind. Eng. Chem. Res., 43(23), 7227 (2004)
Abanades JC, Alvarez D, Energy Fuels, 17(2), 308 (2003)
