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Received March 13, 2014
Accepted December 9, 2014
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Effective adsorption of phenols using nitrogen-containing porous activated carbon prepared from sunflower plates
Zhengguo Zhang
Xiaoqin Feng
Xiao-Xia Yue
Fu-Qiang An†
Wen-Xia Zhou
Jian-Feng Gao
Tuo-Ping Hu†
Chin-Chuan Wei1
Chemical Department, North University of China, Taiyuan 030051, P. R. China 1Biochemistry/Biophysics, Southern Illinois University Edwardsville, USA
anfuqiang@nuc.edu.cn
Korean Journal of Chemical Engineering, August 2015, 32(8), 1564-1569(6), 10.1007/s11814-014-0372-0
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Abstract
Nitrogen-containing porous carbons, the 800SP-NH3, were synthesized using sunflower plates as the major carbon source carbonized at 800 oC and activated with concentrated aqueous ammonia at the same temperature. The porous carbons were characterized by nitrogen physical adsorption-desorption, surface area analyzer, FT-IR, and SEM. The adsorption properties of the porous carbons towards phenols were also investigated by batch methods. The test results show that the average pore diameter of porous carbon is smaller than 2 nm, and nitrogen-containing chemical groups are formed on its surface. The adsorption capacity for phenol, 4-chlorophenol, and p-nitrophenol is 316.5mg/g, 330.24mg/g and 387.62mg/g due to its developed pore structure and nitrogen-containing chemical groups. The adsorption isotherm data greatly obey the Langmuir model.
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