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Received January 17, 2015
Accepted May 30, 2015
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Electrochemical degradation of the Acid Orange 10 dye on a Ti/PbO2 anode assessed by response surface methodology
Gholamreza Bonyadinejad
Mansour Sarafraz
Mohsen Khosravi1
Afshin Ebrahimi†
Seyed Mahmood Taghavi-Shahri2
Roya Nateghi
Sedighe Rastaghi3
Environment Research Center and Department of Environmental Health Engineering, School of Health, Isfahan University of Medical Sciences, Isfahan 81676-36954, Iran 1Nanotechnology Department, University of Isfahan, Isfahan 81744-73441, Iran 2Research Center for Environmental Pollutants, Qom University of Medical Sciences, Qom 37136-49373, Iran 3Department of Epidemiology and Biostatistics, School of Health, Isfahan University of Medical Sciences, Isfahan 81676-36954, Iran
a_ebrahimi@hlth.mui.ac.ir
Korean Journal of Chemical Engineering, January 2016, 33(1), 189-196(8), 10.1007/s11814-015-0115-x
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Abstract
The decolorization and degradation of the synthetic aqueous solution of the Acid Orange 10 (AO10) dye on Ti/PbO2 anode were investigated using the response surface methodology based on central composite design with three variables: current density, pH, and supporting electrolyte concentration. The Ti/PbO2 electrode was prepared by the electrochemical deposition method. The optimum conditions for AO10 decolorization in synthetic dye solution were electrolyte concentration of 117.04 mM, pH of 12.05, and current density of 73.64 mA cm.2. The results indicated that the most effective factor for AO10 degradation was current density. Furthermore, the color removal efficiency significantly increased with increasing current density. To measure AO10 mineralization under optimum conditions, the chemical oxygen demand (COD) and total organic carbon (TOC) removal were evaluated. Under these conditions, decolorization was completed and 63% removal was recorded for COD and 60% for TOC after 100 min of electrolysis.
Keywords
References
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Martinez-Huitle CA, Brillas E, Appl. Catal. B: Environ., 87(3-4), 105 (2009)
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Rodgers JD, Jedral W, Bunce NJ, Environ. Sci. Technol., 33, 1453 (1999)
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Xu H, Li AP, Qi Q, Jiang W, Sun YM, Korean J. Chem. Eng., 29(9), 1178 (2012)
Aquino JM, Pereira GF, Rocha RC, Bocchi N, Biaggio SR, J. Hazard. Mater., 192(3), 1275 (2011)
Murphy OJ, Hitchens GD, Kaba L, Verostko CE, Water Res., 26, 443 (1992)
Vlyssides A, Loizidou M, Karlis P, Zorpas A, Papaioannou D, J. Hazard. Mater., 70, 41 (1999)
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Efron B, Gong G, J. Am. Stat. Assoc., 37, 36 (1983)
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Zhang C, Jiang YH, Li YL, Hu ZX, Zhou L, Zhou MH, Chem. Eng. J., 228, 455 (2013)
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Shao D, Liang JD, Cui XM, Xu H, Yan W, Chem. Eng. J., 244, 288 (2014)
Alvarez-Guerra E, Dominguez-Ramos A, Irabien A, Chem. Eng. Res. Des., 89(12A), 2679 (2011)
