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Received March 24, 2015
Accepted August 8, 2015
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Adsorption properties of Friedel’s salt for the nitrate in the landfill
1College of Life Science, Taizhou University, Linhai 317000, China 2Department of Environmental Engineering, Zhejiang University, Hangzhou 310029, China 3, China 4Zhejiang Provincial Key Laboratory of Solid Waste Treatment and Recycling, Zhejiang Gongshang University, Hangzhou 310018, China
Korean Journal of Chemical Engineering, February 2016, 33(2), 553-558(6), 10.1007/s11814-015-0174-z
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Abstract
Adsorption characteristics of nitrate on Friedel’s salt under the landfill circumstance were investigated to explore the effect of Friedel’s salt on the migration of nitrate in the landfill. Friedel’s salt was synthesized by a coprecipitation method and characterized by XRD and FTIR spectroscopy. The kinetics and isotherm of the adsorption were studied. The effect of the variation of landfill circumstance on the adsorption was also discussed. The result showed that the adsorption capacity of Friedel’s salt for nitrate was 2.494mg g.1. The adsorption process was exothermic and could be well described by pseudo-second-order kinetics and Langmuir-Freundlich equation. Cl. could enhance the adsorption, while SO4 2., PO4 3. and organic matter could restrict the adsorption. The results suggested that the migration of nitrate in the landfill could be altered by Friedel’s salt, which was related to the variation of the landfill circumstance.
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References
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Yao J, Kong QN, Zhu HY, Long YY, Shen DS, Chem. Eng. J., 254, 479 (2014)
Wu YY, Chi Y, Bai HM, Qian GR, Cao YL, Zhou JZ, Xu YF, Lu Q, Xu ZP, Qiao SZ, J. Hazard. Mater., 176(1-3), 193 (2010)
Kjeldsen P, Barlaz MA, Rooker AP, Baun A, Ledin A, Christensen TH, Crit. Rev. Environ. Sci. Technol., 32, 297 (2002)
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Kumar M, Tripathi BP, Shahi VK, J. Hazard. Mater., 172(2-3), 1041 (2009)
Xiao X, Tian F, Yan Y, Wu Z, Cravotto G, Korean J. Chem. Eng., 32(6), 1129 (2015)
Periasamy K, Namasivayam C, Ind. Eng. Chem. Res., 33(2), 317 (1994)
Bayramoglu G, Altintas B, Arica MY, Chem. Eng. J., 152(2-3), 339 (2009)
Shen CS, Shen Y, Wen YZ, Wang HY, Liu WP, Water Res., 45, 5200 (2011)
Wan DJ, Liu HJ, Liu RP, Qu JH, Li SS, Zhang J, Chem. Eng. J., 195-196, 241 (2012)
Hamoudi S, Belkacemi K, Fuel, 110, 107 (2013)
Ganesan P, Kamaraj R, Vasudevan S, J. Taiwan. Inst. Chem. E., 44, 808 (2013)
Islam M, Patel R, J. Hazard. Mater., 190(1-3), 659 (2011)
Ozturk N, Bektas TE, J. Hazard. Mater., 112(1-2), 155 (2004)
Costa DG, Rocha AB, Souza WF, Chiaro SSX, Leitao AA, Appl. Clay Sci., 56, 16 (2012)
Miyata S, Clay. Clay Miner., 31, 305 (1983)
