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- In relation to this article, we declare that there is no conflict of interest.
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Received June 18, 2015
Accepted November 26, 2015
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This is an Open-Access article distributed under the terms of the Creative Commons Attribution Non-Commercial License (http://creativecommons.org/licenses/bync/3.0) which permits
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Preparation of mixed matrix PES-based nanofiltration membrane filled with PANI-co-MWCNT composite nanoparticles
Department of Chemical Engineering, Faculty of Engineering, Arak University, Arak 38156-8-8349, Iran
a.moghadassi@gmail.com, a-moghadassi@araku.ac.ir
Korean Journal of Chemical Engineering, April 2016, 33(4), 1462-1471(10), 10.1007/s11814-015-0257-x
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Abstract
Mixed matrix polyethersulfone/PANI-co-MWCNTs composite nanoparticle nanofiltration membrane was prepared by casting solution technique. Polyvinylpyrrolidone was also used as membrane pore former in membrane fabrication. The effect of polyaniline-co-multi walled carbon nanotubes composite nanoparticle concentration in the casting solution on membrane structure and performance was investigated. Scanning optical microscopy and scanning electron microscopy, FTIR analysis, porosity, mean pore size, contact angle, water content, NaCl/Na2SO4 rejection, water flux, tensile strength measurements and 3D surface image were also carried out in membrane characterization. SOM images showed nanoparticle agglomeration at high additive loading ratio. SEM images showed the membrane sub-layer porosity and thickness were changed by use of nanoparticles in membrane matrix. The membrane water content, porosity and pore size were increased by increase of nanoparticle concentration, except for 1%wt. Use of PANI-co-MWCNT nanoparticles in the membrane matrix caused a decrease of membrane contact angle from 63.43 to 46.76o. Salt rejection and water flux were improved initially by increase of nanoparticle concentration up to 0.1%wt and then decreased by more additive concentration. In addition, the membranes tensile strength was reduced by increase of PANI-co-MWCNTs composite nanoparticle concentration. 3D surface images showed a smoother surface for mixed matrix membrane filled with 0.1wt% PANI-co-MWCNTs. Modified membrane containing 0.1wt% composite nanoparticles showed better performance compared to others.
Keywords
References
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Cho CH, Oh KY, Kim SK, Yeo JG, Sharma P, J. Membr. Sci., 371(1-2), 226 (2011)
Eriksson P, J. Membr. Sci., 36, 297 (1988)
Simpson AE, Kerr CA, Buckley CA, Desalination, 64, 305 (1987)
Cadotte JE, Forester F, Kim M, Petersen RJ, Stocker T, Desalination, 70, 77 (1988)
Raman LP, Cheryan M, Rajagopalan N, Chem. Eng. Prog., 90(3), 68 (1994)
Petersen RJ, J. Membr. Sci., 83, 81 (1993)
Du RH, Zhao JS, J. Membr. Sci., 239(2), 183 (2004)
Mulder M, Basic Principles of Membrane Technology, Kluwer Academic Publishers, Dordrecht (1997).
Ghaemi N, Madaeni SS, Alizadeh A, Daraei P, Vatanpour V, Falsafi M, Desalination, 290, 99 (2012)
Kesting RE, Synthetic Polymeric Membranes, Wiley, New York (1985).
Maximous N, Nakhla G, Wan W, Wong K, J. Membr. Sci., 341(1-2), 67 (2009)
Liu F, Hashim NA, Liu YT, Abed MRM, Li K, J. Membr. Sci., 375(1-2), 1 (2011)
Khodabakhshi AR, Madaeni SS, Hosseini SM, Polym. Int., 60, 466 (2011)
Zendehnam A, Arabzadegan M, Hosseini SM, Robatmili N, Madaeni SS, Korean J. Chem. Eng., 30(6), 1265 (2013)
Zendehnam A, Rabieyan M, Hosseini SM, Mokhtari S, Korean J. Chem. Eng., 32(3), 501 (2015)
Kogure M, Ohya H, Paterson R, Hosaka M, Kim JJ, Mcfadzean S, J. Membr. Sci., 126(1), 161 (1997)
Ohya H, Masaoka K, Aihara M, Negishi Y, J. Membr. Sci., 146(1), 9 (1998)
Thomassin JM, Kollar J, Caldarella G, Germain A, Jerome R, Detrembleur C, J. Membr. Sci., 303(1-2), 252 (2007)
Sabzi RE, Rezapour K, Samadi N, J. Serb. Chem. Soc., 75(4), 537 (2010)
Wang G, Ding Y, Wang F, Li X, Li C, J. Colloid Interface Sci., 317(1), 199 (2008)
Mansour MS, Ossman ME, Farag HA, Desalination, 272(1-3), 301 (2011)
Khan AA, Paquiza L, Desalination, 265(1-3), 242 (2011)
Liu P, Eur. Polym. J., 41, 2693 (2005)
Daraei P, Madaeni SS, Ghaemi N, Monfared HA, Khadivi MA, Sep. Purif. Technol., 104, 32 (2013)
Oueiny C, Berlioz S, Perrin FX, Prog. Polym. Sci, http://dx.doi.org/10.1016/j.progpolymsci.2013.08.009. (2014)
Li XF, Wang Z, Lu H, Zhao CJ, Na H, Zhao C, J. Membr. Sci., 254(1-2), 147 (2005)
Hosseini SM, Hamidi A, Moghadassi A, Madaeni SS, Korean J. Chem. Eng., 32(3), 429 (2015)
Vatanpour V, Madaeni SS, Moradian R, Zinadini S, Astinchap B, Sep. Purif. Technol., 90, 69 (2012)
Hamid NAA, Ismail AF, Matsuura T, Zularisam AW, Lau WJ, Yuliwati E, Abdullah MS, Desalination, 273(1), 85 (2011)
Van der Bruggen B, J. Appl. Polym. Sci., 114(1), 630 (2009)
Mandal MK, Dutta S, Bhattacharya PK, Chem. Eng. J., 138(1-3), 10 (2008)
Han RL, Zhang SH, Liu C, Wang YT, Jian XG, J. Membr. Sci., 345(1-2), 5 (2009)
Gholami A, Moghadassi AR, Hosseini SM, Shabani S, Gholami F, J. Ind. Eng. Chem., 20(4), 1517 (2014)
Ghaemi N, Madaeni SS, Daraei P, Rajabi H, Shojaeimehr T, Rahimpour F, Shirvani B, J. Hazard. Mater., 298, 111 (2015)
Vatanpour V, Madaeni SS, Moradian R, Zinadini S, Astinchap B, J. Membr. Sci., 375(1-2), 284 (2011)
Ansari S, Moghadassi AR, Hosseini SM, Desalination, 357, 189 (2015)
Hosseini SM, Jeddi F, Nemati M, Madaeni SS, Moghadassi AR, Desalination, 341, 107 (2014)
Le-Clech P, Chen V, Fane TAG, J. Membr. Sci., 284(1-2), 17 (2006)
Rana D, Matsuura T, Chem. Rev., 110(4), 2448 (2010)
Daraei P, Madaeni SS, Ghaemi N, Salehi E, Khadivi MA, Moradian R, Astinchap B, J. Membr. Sci., 415, 250 (2012)
Mobarakabad P, Moghadassi AR, Hosseini SM, Desalination, 365, 227 (2015)
Qiu S, Wu LG, Pan XJ, Zhang L, Chen HL, Gao CJ, J. Membr. Sci., 342(1-2), 165 (2009)
