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Received September 7, 2015
Accepted January 25, 2016
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This is an Open-Access article distributed under the terms of the Creative Commons Attribution Non-Commercial License (http://creativecommons.org/licenses/bync/3.0) which permits
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A novel CCU approach of CO2 by the system 1,2-ethylenediamine+1,2-ethylene glycol
College of Chemical Engineering, Inner Mongolia University of Technology, Huhhot 010051, China
tadzhang@pku.edu.cn
Korean Journal of Chemical Engineering, June 2016, 33(6), 1883-1888(6), 10.1007/s11814-016-0023-8
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Abstract
As a new, effective CO2 fixation system, 1,2-ethylenediamine and 1,2-ethylene glycol (EDA+EG) can efficiently activate CO2 and directly convert it into a novel CO2-storage material (CO2SM) with 46.3% yield. The aqueous CO2SM solution can react with Ca(OH)2-saturated limpid solution to generate morphology-controllable CaCO3 microparticles with additional CO2 bubbling and Ca(OH)2. Additionally, the aqueous EDA+EG solution could be recycled multiple times without significant loss of CO2 capturing and releasing capabilities.
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References
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Li FF, Yang ZH, Zeng R, Yang G, Chang X, Yan JB, Hou YL, Ind. Eng. Chem. Res., 50(10), 6496 (2011)
Zaman M, Lee JH, Korean J. Chem. Eng., 30(8), 1497 (2013)
Ma SC, Chen GD, Han TT, Zhu SJ, Yang J, Int. J. Greenh. Gas Con., 37, 249 (2015)
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Goeppert A, Czaun M, Prakash GKS, Olah GA, Energy Environ. Sci., 5, 7833 (2012)
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Barbarossa V, Barzagli F, Mani F, Lai S, Stoppioni P, Vanga G, RSC Adv., 3, 12349 (2013)
Sathre R, Chester M, Cain J, Masanet E, Energy, 37(1), 540 (2012)
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Jin HG, Gao L, Han W, Hong H, Energy, 35(11), 4499 (2010)
Sculley JP, Zhou HC, Angew. Chem.-Int. Edit., 51, 12660 (2012)
Bonenfant D, Mimeault M, Hausler R, Ind. Eng. Chem. Res., 42(14), 3179 (2003)
Camper D, Bara JE, Gin DL, Noble RD, Ind. Eng. Chem. Res., 47(21), 8496 (2008)
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Wang T, Jens K, Int. J. Greenh. Gas Con., 37, 354 (2015)
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Takeda Y, Okumura S, Sasaki I, Minakata S, Org Lett., 14, 4874 (2012)
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Gouedard C, Picq D, Launay F, Carrette PL, Int. J. Greenh. Gas Con., 10, 244 (2012)
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Liu Y, Jessop PG, Cunningham MF, Eckert CA, Liotta CL, Science, 313, 958 (2006)
Kim M, Park J, Chem. Commun., 46, 2507 (2010)
Klimaszewski K, Borun A, Bald A, Sengwa RJ, J. Chem. Eng. Data, 57(11), 3164 (2012)
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Li J, You CJ, Chen LF, Ye YM, Qi ZW, Sundmacher K, Ind. Eng. Chem. Res., 51(37), 12081 (2012)
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Shang JP, Liu SM, Ma XY, Lu LJ, Deng YQ, Green Chem., 14, 2899 (2012)
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Srikanth CS, Chuang SSC, J. Phys. Chem. C, 117, 9196 (2013)
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Barzagli F, Mani F, Peruzzini M, Energy Environ. Sci., 2, 322 (2009)
Enrico A, Eoghan PD, Laurie C, Lawrence BA, Andrew RB, Sci. Rep., 4, 7304 (2014)
Heldebrant DJ, Yonker CR, Jessop PG, Phan L, Energy Environ. Sci., 1, 487 (2008)
Packer M, Energy Policy, 37(9), 3428 (2009)
