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- In relation to this article, we declare that there is no conflict of interest.
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Received May 23, 2017
Accepted August 9, 2017
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Plasmon-enhanced ZnO nanorod/Au NPs/Cu2O structure solar cells: Effects and limitations
Il-Han Yoo
Shankara Sharanappa Kalanur
Kiryung Eom
Byungmin Ahn
In Sun Cho
Hak Ki Yu
Hyeongtag Jeon1†
Hyungtak Seo†
Department of Energy Systems Research and Department of Materials Science & Engineering, Ajou University, Suwon 16499, Korea 1Division of Materials Science & Engineering, Hanyang University, Seoul 04763, Korea
Korean Journal of Chemical Engineering, December 2017, 34(12), 3200-3207(8), 10.1007/s11814-017-0222-y
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Abstract
Cu-based compounds can be a good candidate for a low cost solar cell material. In particular, CuxO (x : 1- 2) has a good visible light absorbing bandgap at 1-2 eV. As for using nanostructures in solar cell applications, metal nanoparticle-induced localized plasmon resonance is a promising way to increase light absorbance, which can help improve the efficiency of solar cells. We fabricated ZnO nanorod/Au nanoparticles/Cu2O nanostructures to study their solar cell performance. ZnO nanorods and Cu2O layer were synthesized by the electrodeposition method. Size-controlled Au nanoparticles were deposited using E-beam evaporator for localized surface plasmon resonance (LSPR) effect. By inserting Au plasmon nanoparticles and annealing Au NPs in solar cells, we could tune the maximum incident photon-to-current efficiency wavelength. However, the potential well formed by Au NP at the ZnO/Cu2O junction leads to charge-trapping, based on the constructed electronic band analysis. LSPR-induced hot carrier generation is proposed to promote carrier transport further in the presence of Au NPs.
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References
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Mittiga A, Salza E, Sarto F, Tucci M, Vasanthi R, Appl. Phys. Lett., 88, 163502 (2006)
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Mattox TM, Ye XC, Manthiram K, Schuck PJ, Alivisatos AP, Urban JJ, Adv. Mater., 27(38), 5830 (2015)
Ren S, Wang B, Zhang H, Ding P, Wang Q, ACS Appl. Mater. Interfaces, 7, 4066 (2015)
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Kraut EA, Grant RW, Waldrop JR, Kowalczyk SP, Phys. Rev. B, 28, 1965 (1983)
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Yoo IH, Kalanur SS, Lee SY, Eom K, Jeon H, Seo H, RSC Adv., 6, 82900 (2016)
Platzer-Bjorkman C, Frisk C, Larsen JK, Ericson T, Li SY, Scragg JJS, Keller J, Larsson F, Torndahl T, Appl. Phys. Lett., 107, 243904 (2015)
Hao X, Sun K, Yan C, Liu F, Huang J, Pu A, et al., In:Photovoltaic Specialists Conference (PVSC), 2016 IEEE 43rd: IEEE, 2016; 2164-2168.
Zheng X, Chen B, Yang M, Wu C, Orler B, Moore RB, et al., ACS Energy Lett., 1, 424 (2016)
Yoon K, Hyun JK, Connell JG, Amit I, Rosenwaks Y, Lauhon LJ, Nano Lett., 13, 6183 (2013)
