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Received July 15, 2016
Accepted November 5, 2016
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This is an Open-Access article distributed under the terms of the Creative Commons Attribution Non-Commercial License (http://creativecommons.org/licenses/bync/3.0) which permits
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CO2 capture performance of cement-modified carbide slag
School of Energy and Power Engineering, Shandong University, Jinan 250061, China 1State Key Laboratory of Crystal Materials, Shandong University, Jinan 250100, China
Korean Journal of Chemical Engineering, February 2017, 34(2), 580-587(8), 10.1007/s11814-016-0315-z
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Abstract
A novel and low-cost synthetic CO2 sorbent for calcium looping process, cement-modified carbide slag (CMCS), was synthesized from carbide slag, aluminate cement and by-product of biodiesel by combustion. The effects of synthesis conditions such as combustion temperature, combustion duration, hydration, by-product of biodiesel and cement addition and regeneration temperature on CO2 capture performance of CMCS were investigated. The comprehensively optimum preparation conditions of CMCS were obtained. The highest CO2 capture capacity is 0.62 g/g after 10 cycles, which is 2.18 times as high as that of carbide slag. The addition of aluminate cement improves the CO2 capture performance of CMCS, while excessive aluminate cement is adverse for CO2 capture due to the reduced CaO content in CMCS. The addition of by-product of biodiesel contributes to a uniform sol mixing of carbide slag and cement. The CMCS exhibits higher carbonation and calcination rates than CS. The porous and stable pore structure leads to the better CO2 capture performance and cyclic stability of CMCS.
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