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- In relation to this article, we declare that there is no conflict of interest.
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Received February 12, 2017
Accepted March 16, 2017
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This is an Open-Access article distributed under the terms of the Creative Commons Attribution Non-Commercial License (http://creativecommons.org/licenses/bync/3.0) which permits
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Fabrication of sensory structure based on poly (ethylene glycol)-diacrylate hydrogel embedding polydiacetylene
1Department of Chemical and Biological Engineering, Korea University, Seoul 02841, Korea 2KU-KIST Graduate School of Converging Science and Technology, Korea University, Seoul 02841, Korea
ahn@korea.ac.kr
Korean Journal of Chemical Engineering, July 2017, 34(7), 2092-2095(4), 10.1007/s11814-017-0083-4
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Abstract
Hydrogel-based sensory structures were developed by embedding polydiacetylene supramolecules into poly-(ethylene glycol)-diacrylate (PEG-DA) to detect chemical gases and cyclodextrin and to determine pH values on the basis of a fluorescence change. We found the optimal condition for patterning-fabrication by controlling the volumetric mixture ratio of the water-soluble PEG-DA and aqueous polydiacetylene vesicle solution. Then, we determined that this hydrogel-based polydiacetylene structure optically responded selectively against vapor-phase targets: ammonia, ethanol, and aldehyde; aqueous solutions with various pH values; and cyclodextrin derivatives. These results could be extended to various label-free sensing applications of hydrogel-based chemo-biosensors.
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References
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Kew SJ, Hall EAH, Anal. Chem., 78, 2231 (2006)
Giokas DL, Vlessidis AG, Anal. Chim. Acta, 683, 156 (2011)
Peppas NA, Hilt JZ, Khademhosseini A, Langer R, Adv. Mater., 18(11), 1345 (2006)
Lee KY, Mooney DJ, Chem. Rev., 101(7), 1869 (2001)
Mellott MB, Searcy K, Pishko MV, Biomaterials, 22, 929 (2001)
Schmidt T, Monch JI, Arndt KF, Macromol. Mater. Eng., 291, 755 (2006)
Asoh TA, Matsusaki M, Kaneko T, Akashi M, Adv. Mater., 20(11), 2080 (2008)
Witte RP, Blake AJ, Palmer C, Kao WJ, J. Biomed. Mater. Res., 71A, 508 (2004)
Hahn MS, Taite LJ, Moon JJ, Rowland MC, Ruffino KA, West JL, Biomaterials, 27, 2519 (2006)
Hahn MS, Miller JS, West JL, Adv. Mater., 18(20), 2679 (2006)
Cho BW, Kim DH, Lee HW, Na BK, Korean J. Chem. Eng., 24(6), 1037 (2007)
Moon JJ, Hahn MS, Kim I, Nsiah BA, West JL, Tissue Eng., 15, 579 (2008)
Sui ZJ, King WJ, Murphy WL, Adv. Funct. Mater., 18(12), 1824 (2008)
Wu YH, Park HB, Kai T, Freeman BD, Kalika DS, J. Membr. Sci., 347(1-2), 197 (2010)
Okada SY, Jelinek R, Charych D, Angew. Chem.-Int. Edit., 38, 655 (1999)
Shim HY, Lee SH, Ahn DJ, Ahn K, Kim JM, Mater. Sci. Eng. C,, 24, 157 (2004)
Kim JM, Lee J, Lee J, Woo S, Ahn DJ, Macromol. Chem. Phys., 206, 2299 (2005)
Kim JM, Lee YB, Yang DH, Lee JS, Lee GS, Ahn DJ, J. Am. Chem. Soc., 127(50), 17580 (2005)
Kim JM, Chae SK, Lee YB, Lee JS, Lee GS, Kim TY, Ahn DJ, Chem. Lett., 35(6), 560 (2006)
Ahn DJ, Kim JM, Acc. Chem. Res., 41, 805 (2008)
Park S, Lee GS, Cui C, Ahn DJ, Macromol. Res., 24(4), 380 (2016)
Hyun JY, Lee GS, Kim TY, Ahn DJ, Korean J. Chem. Eng., 14(6), 533 (1997)
Ji EK, Ahn DJ, Kim JM, B. Korean. Chem. Soc., 24, 667 (2003)
Kwak SK, Lee GS, Ahn DJ, Choi JW, Mat. Sci. Eng. C, 24, 151 (2004)
Kim KW, Choi H, Lee GS, Ahn DJ, Oh MK, Kim JM, Macromol. Res., 14(4), 483 (2006)
Kim KW, Choi H, Lee GS, Ahn DJ, Oh M, Colloids Surf. B: Biointerfaces, 66, 213 (2008)
Charoenthai N, Pattanatornchai T, Wacharasindhu S, Sukwattanasinitt M, Traiphol R, J. Colloid Interface Sci., 360(2), 565 (2011)
Tachibana H, Hosaka N, Tokura Y, Polymer, 42(19), 8311 (2001)
Kew SJ, Hall EAH, Anal. Chem., 78, 2231 (2006)
Giokas DL, Vlessidis AG, Anal. Chim. Acta, 683, 156 (2011)
