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Received March 4, 2018
Accepted June 24, 2018
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This is an Open-Access article distributed under the terms of the Creative Commons Attribution Non-Commercial License (http://creativecommons.org/licenses/bync/3.0) which permits
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Carbon dioxide reforming of methane over MgO promoted Ni/CNT catalyst
Dehua Zhang
Guangcheng Wei
Yiru Wang
Jing Wang
Ping Ning
Qiulin Zhang†
Mingzhi Wang
Tengfei Zhang
Kaixian Long
Faculty of Environmental Science and Engineering, Kunming University of Science and Technology, Kunming 650500, P. R. China
qiulinzhang_kmust@163.com
Korean Journal of Chemical Engineering, October 2018, 35(10), 1979-1987(9), 10.1007/s11814-018-0108-7
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Abstract
Carbon dioxide reforming of methane to syngas was investigated over a series of MgO promoted Ni/CNT catalysts. MgO played a critical role in improving the catalytic performance of Ni/CNT. The results showed that the addition of MgO strengthened the interaction of Ni and interior surface of CNT. Highly dispersed nickel particles with small size (less than 4.5 nm) were also observed in MgO modified CNT. Otherwise, the NiO nanoparticles were facilely reduced over the catalyst prepared with a narrow size of CNT, as shown in H2-TPR. The reaction tests demonstrated that the Ni-based catalyst with an addition of MgO and narrow size of CNT exhibited better catalytic activity. Furthermore, the lifetime of Ni-based catalyst was prolonged effectively after adding MgO, attributed to the stabilization and dispersion of Ni particles and the effective restraint on the gasification of CNT.
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