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Received April 22, 2018
Accepted September 27, 2018
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Facile synthesis of ZnBi2O4-graphite composites as highly active visible-light photocatalyst for the mineralization of rhodamine B
Nguyen Thi Mai Tho1 2
Bui The Huy3 4†
Dang Nguyen Nha Khanh5
Ho Nguyen Nhat Ha5
Vu Quang Huy5
Ngo Thi Tuong Vy6
Do Manh Huy7
Duong Phuoc Dat7
Nguyen Thi Kim Phuong1 5†
1Graduate University of Science and Technology, Vietnam Academy of Science and Technology (VAST), 18 Hoang Quoc Viet, Cau Giay, Hanoi, Vietnam 2Chemical Engineering Faculty, Industrial University of Ho Chi Minh City, Vietnam 3**Institute of Research and Development, Duy Tan University, 03 Quang Trung, Da Nang, Vietnam 4Department of Chemistry, Changwon National University, Changwon 51140, Korea 5HoChiMinh City Institute of Resources Geography, VAST, 01 Mac Dinh Chi, Ho Chi Minh City, Vietnam 6University of Science, National University of Ho Chi Minh City, Vietnam 7Institute of Chemical Technology, VAST, 01 Mac Dinh Chi, Ho Chi Minh City, Vietnam
Korean Journal of Chemical Engineering, December 2018, 35(12), 2442-2451(10), 10.1007/s11814-018-0156-z
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Abstract
Novel highly active visible-light photocatalysts in the form of zinc bismuth oxide (ZnBi2O4) and graphite hybrid composites were prepared by coupling via a co-precipitation method followed by calcination at 450 °C. The asprepared ZnBi2O4-graphite hybrid composites were tested for the degradation of rhodamine B (RhB) solutions under visible-light irradiation. The existence of strong electronic coupling between the two components within the ZnBi2O4- graphite heterostructure suppressed the photogenerated recombination of electrons and holes to a remarkable extent. The prepared composite exhibited excellent photocatalytic activity, leading to more than 93% of RhB degradation at an initial concentration of 50mgㆍL-1 with 1.0 g catalyst per liter in 150min. The excellent visible-light photocatalytic mineralization of ZnBi2O4-1.0graphite in comparison with pristine ZnBi2O4 could be attributed to synergetic effects, charge transfer between ZnBi2O4 and graphite, and the separation efficiency of the photogenerated electrons and holes. The photo-induced h+ and the superoxide anion were the major active species responsible for the photodegradation process. The results demonstrate the feasibility of ZnBi2O4-1.0graphite as a potential heterogeneous photocatalyst for environmental remediation.
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Zhang SQ, Yang YX, Guo YN, Guo W, Wang M, Guo YH, Huo MX, J. Hazard. Mater., 261, 235 (2013)
