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Received April 27, 2018
Accepted September 18, 2018
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Investigation of short-term stability in high efficiency polymer : nonfullerene solar cells via quick current-voltage cycling method
1*Organic Nanoelectronics Laboratory and KNU Institute for Nanophotonics Applications (KINPA), Department of Chemical Engineering, School of Applied Chemical Engineering, Kyungpook National University, Daegu 41566, Korea 2Research Institute of Advanced Energy Technology, Kyungpook National University, Daegu 41566, Korea 3Polymer Rheology Laboratory, Department of Chemical Engineering, School of Applied Chemical Engineering,, Kyungpook National University, University Road 80, Daegu 41566, Korea
khj217@knu.ac.kr
Korean Journal of Chemical Engineering, December 2018, 35(12), 2496-2503(8), 10.1007/s11814-018-0154-1
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Abstract
The short-term stability of high efficiency polymer : nonfullerene solar cells was investigated by employing a quick (ten cycles) current density-voltage (J-V) cycling method. Polymer : nonfullerene solar cells with initial power conversion efficiency (PCE) of >10% were fabricated using bulk heterojunction (BHJ) films of poly[(2,6-(4,8-bis(5-(2- ethylhexyl)thiophen-2-yl)-benzo[1,2-b:4,5b']dithiophene))-alt-(5,5-(1',3'-di-2-thienyl-5,7'-bis(2-ethylhexyl)benzo[1',2'- c:4',5'-c']dithiophene-4,8-dione))] (PBDB-T) and 3,9-bis(2-methylene-((3-(1,1-dicyanomethylene)-6/7-methyl)-indanone))- 5,5,11,11-tetrakis(4-hexylphenyl)-dithieno[2,3-d:2',3'-d']-s-indaceno[1,2-b:5,6-b']dithiophene (IT-M). One set of the BHJ (PBDB-T : IT-M) films was thermally annealed at 160 °C for 30min, while another set was used without any thermal treatment after spin-coating. The quick J-V scan (cycling) measurement disclosed that the PCE decay was relatively slower for the annealed BHJ layers than the unannealed (as-cast) BHJ layers. As a result, after ten cycles, the annealed BHJ layers delivered higher PCE than the unannealed BHJ layers due to higher and more stable trend in fill factor. The present quick J-V cycling method is simple but expected to be useful for the prediction of short-term stability in organic solar cells.
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Coropeanu V, Bredas J, J. Phys. Chem. C, 121, 24954 (2017)
Cheng P, Yan CQ, Wu Y, Wang JY, Qin M, An QS, Cao JM, Huo LJ, Zhang FJ, Ding LM, Sun YM, Ma W, Zhan XW, Adv. Mater., 28(36), 8021 (2016)
Serbenta A, Kozlov OV, Portale G, Loosdrecht PHM, Pshenichnikov MS, Sci. Rep., 6, 36236 (2016)
Cheng P, Yan CQ, Lau TK, Mai JQ, Lu XH, Zhan XW, Adv. Mater., 28(28), 5822 (2016)
Huang W, Gann E, Cheng YB, McNeill CR, ACS Appl. Mater. Interfaces, 7, 14026 (2015)
Qin M, Cheng P, Mai J, Lau TK, Zhang Q, Wang J, Yan C, Liu K, Su CJ, You W, Lu X, Zhang X, Sol. RRL, 1, 170014 (2017)
Huang W, Chandrasekaranm N, Prasad SKK, Gann E, Thomsen L, Kabra D, Hodgkiss JM, Cheng YB, McNeill CR, ACS Appl. Mater. Interfaces, 8, 29608 (2016)
Zhang XH, Zheng D, Xing S, Wang HY, Huang J, Yu JS, Sol. Energy, 147, 106 (2017)
Liu F, Chen D, Wang C, Luo K, Gu W, Briseno AL, Hsu JWP, Russell TP, ACS Appl. Mater. Interfaces, 6, 19876 (2014)
Li SS, Ye L, Zhao WC, Zhang SQ, Mukherjee S, Ade H, Hou JH, Adv. Mater., 28(42), 9423 (2016)
Hwang YJ, Li HY, Courtright BAE, Subramaniyan S, Jenekhe SA, Adv. Mater., 28(1), 124 (2016)
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Ma Y, Zhang M, Tang Y, Ma W, Zheng Q, Chem. Mater., 29, 9775 (2017)
Park G, Choi S, Park S, Lee D, Cho M, Choi D, Adv. Energy Mater., 7, 170056 (2017)
Cheng P, Bai H, Zawacka NK, Anderson TR, Liu W, Bundgaard E, Jorgensen M, Chen H, Krebs FC, Zhan X, Adv. Sci., 2, 150009 (2015)
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Chambon S, Rivaton A, Gardette JL, Firon M, Polym. Degrad. Stabil., 96, 1149 (2011)
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Grisorio R, Allegretta G, Mastrorilli P, Suranna GP, Macromolecules, 44(20), 7977 (2011)
Zhao W, Li S, Zhang S, Liu X, Hou J, Adv. Mater., 29, 160405 (2016)
Li S, Ye L, Zhao W, Liu X, Zhu J, Ade H, Hou J, Adv. Mater., 29, 170405 (2017)
Guan Q, Peng R, Liu Z, Song W, Yang R, Hong L, Lei T, Wei Q, Ge Z, J. Mater. Chem. A, 6, 464 (2018)
Liu X, Ye L, Zhao W, Zhang S, Li S, Su GM, Wang C, Ade H, Hou J, Mater. Chem. Front., 1, 2057 (2017)
