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Received September 4, 2017
Accepted November 22, 2017
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Removal of Acid Red G dye from aqueous solutions by adsorption to MCM-41-layered double hydroxides composite
State Environmental Protection Key Laboratory of Eco-Industry, Northeastern University, Shenyang 110819, China
dutao2000@hotmail.com
Korean Journal of Chemical Engineering, March 2018, 35(3), 709-716(8), 10.1007/s11814-017-0327-3
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Abstract
MCM-41 supported layered double hydroxides (LDH) composite materials (ML) were synthesized and studied for removal of Acid Red G (ARG), an anionic dye, with the adsorption method. ML was prepared using in situ synthesis procedure for the low supersaturation coprecipitation method, and ML10 and ML20 presented promising application towards ARG dye adsorption capacity in industrial wastewater. Powder samples were characterized by X-ray diffraction, FTIR spectroscopy, scanning electron microscopy and energy dispersive spectrometry. The effects of different reaction time, initial solution pH and temperature on the dye adsorption capacity were investigated. Adsorption process was well described by pseudo-second-order kinetic model and Langmuir isotherm model. The fitting curves showed that ML10 and ML20 had higher adsorption rates and maintained a certain theoretical saturated adsorption capacity (92.19807mg/g and 96.41947mg/g, respectively) compared with LDH.
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Kamboh MA, Solangi IB, Sherazi STH, Memon S, J. Hazard. Mater., 186(1), 651 (2011)
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Jovic-Jovicic N, Milutinovic-Nikolic A, Grzetic I, Jovanovic D, Chem. Eng. Technol., 31(4), 567 (2008)
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Qiu M, Qian C, Xu J, Wu J, Wang G, Desalination, 234, 286 (2009)
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Mohan SV, Rao NC, Karthikeyan J, J. Hazard. Mater., 90(2), 189 (2002)
Janos P, Buchtova H, Ryznarova M, Water Res., 37, 4938 (2003)
Lafi R, Charradi K, Djebbi MA, Amara ABH, Hafiane A, Adv. Powder Technol., 27(1), 232 (2016)
Bayramoglu G, Akbulut A, Liman G, Arica MY, Chem. Eng. Res. Des., 124, 85 (2017)
Parida K, Das J, J. Mol. Catal. A-Chem., 151(1-2), 185 (2000)
Taylor HFW, Mineral. Mag., 39 (1973)
Jiao F, Yu J, Song H, Jiang X, Yang H, Shi S, Chen X, Yang W, Appl. Clay Sci., 101, 30 (2014)
Jia Z, Li S, Liu J, Qin Q, Zhu R, Bull. Mat. Sci., 38, 1757 (2015)
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Kresge CT, Leonowicz ME, Roth WJ, Vartuli JC, Beck JS, Nature, 359, 710 (1992)
Bayramoglu G, Arica MY, Microporous Mesoporous Mater., 226, 117 (2016)
Arica TA, Ayas E, Arica MY, Microporous Mesoporous Mater., 243, 164 (2017)
Lin W, Cai Q, Pang W, Yue Y, Zou B, Microporous Mesoporous Mater., 33, 187 (1999)
Bhatta LKG, Subramanyam S, Chengala MD, Bhatta UM, Venkatesh K, Ind. Eng. Chem. Res., 54(43), 10876 (2015)
Tong DS, Liu M, Li L, Lin CX, Yu WH, Xu ZP, Zhou CH, Appl. Clay Sci., 70, 1 (2012)
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Kushwaha AK, Gupta N, Chattopadhyaya MC, Desalination Water Treat., 52, 4527 (2014)
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Zhang WH, Guo XD, He J, Qian ZY, J. European Ceram. Soc., 28, 1623 (2008)
Lee JM, Min YJ, Lee KB, Jeon SG, Na JG, Ryu HJ, Langmuir, 26(24), 18788 (2010)
Ho YS, J. Hazard. Mater., 136(3), 681 (2006)
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Ahmed IM, Gasser MS, Appl. Surf. Sci., 259, 650 (2012)
de Sa FP, Cunha BN, Nunes LM, Chem. Eng. J., 215, 122 (2013)
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Freundlich HMF, Z. Phys. Chemie-Int. J. Res. Phys. Chem. Chem. Phys., 57ㅁ, 385 (1906)
Langmuir I, J. Am. Chem. Soc., 38, 2221 (1916)
