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- In relation to this article, we declare that there is no conflict of interest.
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Received September 22, 2017
Accepted December 26, 2017
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This is an Open-Access article distributed under the terms of the Creative Commons Attribution Non-Commercial License (http://creativecommons.org/licenses/bync/3.0) which permits
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Anti-fouling characteristic of carbon nanotubes hollow fiber membranes by filtering natural organic pollutants
Key Laboratory of Industrial Ecology and Environmental Engineering (Ministry of Education, China), School of Environmental Science and Technology, Dalian University of Technology, Dalian 116024, P. R. China
Korean Journal of Chemical Engineering, April 2018, 35(4), 964-973(10), 10.1007/s11814-017-0354-0
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Abstract
Membrane fouling is a universal problem for conventional membrane filtration that usually causes a deterioration in membrane performance. We used electro-assisted carbon nanotubes hollow fiber membranes (CNTs-HFMs) to investigate the anti-fouling properties using natural organic pollutants. Benefiting from the electro-assistance, the permeation flux of humic acid solution using CNTs-HFMs was 190.20 L/(m2·h·bar), which was about 1.5- and 4.4- times higher than those of CNTs-HFMs without electro-assistance and traditional polyvinylidene fluoride hollow-fiber membranes (PVDF-HFMs). And the permeation fluxes of bovine serum albumin, sodium alginate and supernatant of anaerobic bioreactor also presented similar results. The average COD removal rate of CNTs-HFMs (66.8%) at .1.0 V was higher than that of CNTs-HFMs without electro-assistance and PVDF-HFMs, which can be attributed to the formation of electrostatic repulsive force. It could reduce the deposition of pollutants on membrane surface under electroassistance.
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References
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Yu M, Funke HH, Falconer JL, Noble RD, Nano Lett., 9, 225 (2008)
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Li QL, Elimelech M, J. Membr. Sci., 278(1-2), 72 (2006)
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Shimizu Y, Rokudai M, Tohya S, Kayawake E, Yazawa T, Kagaku Kogaku Ronbun., 16, 145 (1990)
He ZW, Miller DJ, Kasemset S, Paul DR, Freeman BD, J. Membr. Sci., 525, 25 (2017)
Wang Z, Ci L, Chen L, Nayak S, Aiayan PM, Koratkar N, Nano Lett., 7, 697 (2007)
He B, Patankar NA, Lee J, Langmuir, 19(12), 4999 (2003)
Fan XF, Zhao HM, Liu YM, Quan X, Yu HT, Chen S, Environ. Sci. Technol., 49, 2293 (2015)
Katsoufidou K, Yiantsios SG, Karabelas AJ, J. Membr. Sci., 266(1-2), 40 (2005)
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Contreras AE, Kim A, Li QL, J. Membr. Sci., 327(1-2), 87 (2009)
Kim HC, Dempsey BA, J. Membr. Sci., 428, 190 (2013)
Hashino M, Katagiri T, Kubota N, Ohmukai Y, Maruyama T, Matsuyama H, J. Membr. Sci., 366(1-2), 258 (2011)
Qu F, Liang H, Wang Z, Wang H, Yu H, Li G, Water Res., 46, 1490 (2012)
Bai LM, Liang H, Crittenden J, Qu FS, Ding A, Ma J, Du X, Guo SD, Li GB, J. Membr. Sci., 492, 400 (2015)
Ryssov-Nielsen H, Vatten, 1, 33 (1975)
Novak JT, Zurow A, Becker H, J. Environ. Eng. Div., 103, 815 (1977)
Kang S, Kishimoto M, Shioya S, Yoshida T, Suga K, Taguchi H, J. Ferment. Bioeng., 68, 117 (1989)
Flemming HC, Wingender J, Water Sci. Technol., 43, 1 (2001)
Vatanpour V, Madaeni SS, Moradian R, Zinadini S, Astinchap B, J. Membr. Sci., 375(1-2), 284 (2011)
