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Received August 15, 2017
Accepted December 14, 2017
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Thin film graphene oxide membrane: Challenges and gas separation potential
Department of Petroleum and Chemical Engineering, Sharif University of Technology, Tehran, Iran 1Material and Nuclear Fuel Research School, Nuclear Science and Technology Research Institute, Tehran, Iran
j_karimi@alum.sharif.edu, jvkarimi@aeoi.org.ir
Korean Journal of Chemical Engineering, May 2018, 35(5), 1174-1184(11), 10.1007/s11814-017-0339-z
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Abstract
Graphene oxide membranes were prepared by vacuum and pressurized ultrafiltration methods on the 12% modified Polyacrylonitrile (12mPAN) substrate to specify challenges, salient features, future directions, and potential of GO membrane for separation fields using characterization techniques and gas separation test (studied gases are CO2, He and N2), which is an efficient tool for better understanding of GO membrane behavior. GO membrane structure was examined over a wide range of parameters, such as pore size range of substrate and its surface properties, pH of GO dispersion, GO content, synthesis pressure, operating pressure and temperature. The results show that the GO content does not hold a linear relationship with the permeance and selectivity. Film thickness, aggregates, synthesis pressure defects and interlayer spacing have significant effects on the gas separation performance of GO membranes which originate from the synthesis method and its conditions.
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