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Received March 18, 2018
Accepted May 27, 2018
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A review on metal nitrides/oxynitrides as an emerging supercapacitor electrode beyond oxide
Green Energy Lab., Department of Chemical Engineering, Chungbuk National University, 1 Chungdae-ro, Seowon-gu, Cheongju, Chungbuk 28644, Korea 1Surface and Nanoscience Division, Materials Science Group, Indira Gandhi Centre for Atomic Research, Kalpakkam 603102, India
smjeong@chungbuk.ac.kr
Korean Journal of Chemical Engineering, July 2018, 35(7), 1389-1408(20), 10.1007/s11814-018-0089-6
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Abstract
Electrode materials design is the most significant aspect in constructing a supercapacitor device. The evolution of metal nitrides/oxynitrides as supercapacitor electrode is strikingly noticeable today besides prevailing carbon or 2D materials, metal oxides/hydroxides and conducting polymers electrode materials. The theoretically estimated specific capacitance of a nitride-based supercapacitor is 1,560 F g-1. These nanostructures exhibit an excellent capacitive behavior with a specific capacitance of 15-951.3mF cm-2 or 82-990 F g-1, high energy density (16.5-162Wh Kg-1) and power density (7.3-54,000W Kg-1). On this account, supercapacitor performance of metal nitrides/oxynitrides is reviewed exclusively. The major focus of the present review is directed towards state-of-art progress in supercapacitor performance of nitrides/oxynitrides, underlying charge-storage mechanism, important outcomes and their limitations. Finally, we conclude with challenges and prospects of metal nitrides/oxynitrides for supercapacitor electrodes.
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