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Received February 20, 2018
Accepted April 19, 2018
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This is an Open-Access article distributed under the terms of the Creative Commons Attribution Non-Commercial License (http://creativecommons.org/licenses/bync/3.0) which permits
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Attapulgite/carbon composites as a recyclable adsorbent for antibiotics removal
1Key Laboratory of Clay Mineral Applied Research of Gansu Province, Center of Eco-materials and Green Chemistry, Lanzhou Institute of Chemical Physics, Chinese Academy of Sciences, Lanzhou 730000, P. R. China 2University of Chinese Academy of Sciences, Beijing 100049, P. R. China 3Center of Xuyi Palygorskite Applied Technology, Lanzhou Institute of Chemical Physics, Chinese Academy of Sciences, Xuyi 211700, P. R. China
zongli@licp.cas.cn
Korean Journal of Chemical Engineering, August 2018, 35(8), 1650-1661(12), 10.1007/s11814-018-0066-0
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Abstract
We evaluated the adsorption performance of attapulgite/carbon (APT/C) composite as reusable adsorbents for antibiotics. APT/C composite was first synthesized by one-step calcination based on the spent bleaching earth after bleaching of vegetable oil, and followed by a thermal regeneration after adsorption of antibiotic at different temperatures. Antibiotics adsorption results revealed that APT/C composites prepared at 300 oC exhibited high adsorption capacity and fast equilibrium. Thermal regeneration proved to be an efficient methodology for recycling the spent antibiotic- loaded APT/C composites. After the ten-time continuous adsorption-calcination process, the removal ratios of the recycled adsorbents still retained around 67.3% and 62.9% for chlortetracycline and tetracycline, respectively. The conjugation of the adsorption and regeneration results suggested that combining the advantages of APT and carbon species provided a feasible strategy to fabricate a promising adsorbent with the desirable adsorption and regeneration properties for removal of antibiotics in the future.
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