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Received February 7, 2018
Accepted May 10, 2018
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Interfacial polymerization of facilitated transport polyamide membrane prepared from PIP and IPC for gas separation applications
1Chemical Engineering Department, King Fahd University of Petroleum and Minerals, Dhahran 31261, Saudi Arabia 2Center of Excellence in Nanotechnology, King Fahd University of Petroleum and Minerals, Dhahran 31261, Saudi Arabia
Korean Journal of Chemical Engineering, August 2018, 35(8), 1700-1709(10), 10.1007/s11814-018-0079-8
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Abstract
A facilitated transport polyamide (PA) membrane was developed for gas separation by interfacial polymerization reaction of piperazine (PIP) and isophthaloyl chloride (IPC) supported on polysulfone (PSF) membrane previously prepared by dry/wet phase inversion method. The properties of the prepared membranes were characterized by SEM, FT-IR, TGA, and XRD. SEM images showed that a defect-free PSF, and rough PA membranes were fabricated, while the FT-IR spectra confirmed the formation of PA layer on top of the PSF support. The separation performance of the thin film PA and PSF membranes was evaluated using four gasses (CO2, CH4, N2, and O2). Compared to the PSF membrane, the PA membrane demonstrated an increased selectivity of CO2/CH4 and CO2/N2 by 178%, 169%, respectively. This improvement was attributed to the presence of amine functional groups, which acted as a fixed carrier to facilitate the transport of CO2 gas across the membrane. However, building the PA layer on top of PSF support reduced the membrane permeance of CO2 from 2.41 to 2.12 GPU as a result of the increased mass transfer resistance. Furthermore,_x000D_
the effect of operating temperature and pressure on the separation performance of the membranes was investigated.
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Shimekit B, Mukhtar H, Eds., InTech, Croatia, 235 (2012).
Rezakazemi M, Ebadi A, Prog. Polym. Sci, 39, 817 (2014)
Zhang Y, Sunarso J, Liu S, Wang R, Int. J. Greenh. Gas Control., 12, 84 (2013)
Peters L, Hussain A, Follmann M, Melin T, Hagg MB, Chem. Eng. J., 172(2-3), 952 (2011)
Baker RW, Lokhandwala K, Ind. Eng. Chem. Res., 47(7), 2109 (2008)
Aroon MA, Ismail AF, Matsuura T, Montazer-Rahmati MM, Sep. Purif. Technol., 75(3), 229 (2010)
Zhao J, Wang Z, Wang JX, Wang SC, J. Membr. Sci., 283(1-2), 346 (2006)
Yu XW, Wang Z, Wei ZH, Yuan SJ, Zhao JA, Wang JX, Wang SC, J. Membr. Sci., 362(1-2), 265 (2010)
Yoshikawa M, Fujimoto K, Kinugawa H, Kitao T, Ogata N, Chem. Lett., 23, 243 (1994)
Du RH, Feng XS, Chakma A, J. Membr. Sci., 279(1-2), 76 (2006)
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Matsuyama H, Hirai K, Teramoto M, J. Membr. Sci., 92(3), 257 (1994)
Saedi S, Madaeni SS, Seidi F, Shamsabadi AA, Laki S, Chem. Eng. J., 236, 263 (2014)
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Zhang YF, Xiao C, Liu EH, Du QY, Wang X, Yu HL, Desalination, 191(1-3), 291 (2006)
Li LC, Wang BG, Tan HM, Chen TL, Xu JP, J. Membr. Sci., 269(1-2), 84 (2006)
Shepl Y, Kotp Y, El-deab M, Shawky H, El-anadouli B, J. Membr. Sci., 391, 215 (2012)
Kim JH, Lee KH, Kim SY, J. Membr. Sci., 169(1), 81 (2000)
Zhang Y, Benes NE, Lammertink RGH, AAPG Bull., 15, 575 (2015)
Sridhar S, Smitha B, Mayor S, Prathab B, Aminabhavi TM, J. Mater. Sci., 42(22), 9392 (2007)
Zhang Z, Chen F, Rezakazemi M, Zhang W, Lu C, Chang H, Quan X, Chem. Eng. Res. Des., 131, 375 (2018)
Mo Y, Tiraferri A, Yip NY, Adout A, Huang X, Elimelech M, Environ. Sci. Technol., 46, 13253 (2012)
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Dorosti F, Omidkhah M, Abedini R, J. Nat. Gas Sci. Eng., 25, 88 (2015)
Pesek SC, Koros WJ, J. Membr. Sci., 81, 71 (1993)
Aroon MA, Ismail AF, Montazer-Rahmati MM, Matsuura T, Sep. Purif. Technol., 72(2), 194 (2010)
Chakrabarty B, Ghoshal AK, Purkait AK, J. Membr. Sci., 315(1-2), 36 (2008)
Boom RM, Wlenk IM, Van T, Smolders CA, J. Membr. Sci., 73, 277 (1992)
Ghosh AK, Jeong BH, Huang XF, Hoek EMV, J. Membr. Sci., 311(1-2), 34 (2008)
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Bruck SD, Polymer, 7, 231 (1966)
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Wong KC, Goh PS, Ng BC, Ismail AF, RSC Adv., 5, 31683 (2015)
McDanel WM, Cowan MG, Chisholm NO, Gin DL, Noble RD, J. Membr. Sci., 492, 303 (2015)
Sen SK, Banerjee S, J. Membr. Sci., 350(1-2), 53 (2010)
Bera D, Bandyopadhyay P, Ghosh S, Banerjee S, J. Membr. Sci., 453, 175 (2014)
Banerjee S, Maier G, Dannenberg C, Spinger J, J. Membr. Sci., 229(1-2), 63 (2004)
Li XG, Kresse I, Xu ZK, Springer J, Polymer, 42(16), 6801 (2001)
Xin QP, Wu H, Jiang ZY, Li YF, Wang SF, Li Q, Li XQ, Lu X, Cao XZ, Yang J, J. Membr. Sci., 467, 23 (2014)
Ansaloni L, Zhao YN, Jung BT, Ramasubramanian K, Baschetti MG, Ho WSW, J. Membr. Sci., 490, 18 (2015)
Amooghin AE, Omidkhah M, Kargari A, J. Membr. Sci., 490, 364 (2015)
