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Received April 8, 2018
Accepted May 27, 2018
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Methane combustion over Pd/Ni-Al oxide catalysts: Effect of Ni/Al ratio in the Ni-Al oxide support
Department of Chemical Engineering, Chungbuk National University, Chungbuk 28644, Korea 1Department of Environmental Engineering, Chungbuk National University, Chungbuk 28644, Korea
chshin@chungbuk.ac.kr
Korean Journal of Chemical Engineering, September 2018, 35(9), 1815-1822(8), 10.1007/s11814-018-0090-0
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Abstract
We prepared xNi-2Al oxide (x=0-1.1) supports via a hydrothermal method, and applied Pd/xNi-2Al catalysts in the catalytic methane combustion reaction. It was found that the physicochemical properties of the xNi-2Al supports varied as a function of the Ni content, and the interaction between support and impregnated Pd was also influenced by the Ni content. Furthermore, variation in the Ni content significantly affected the chemical state and reducibility of the impregnated Pd species. Finally, the catalytic activity and stability of prepared Pd/xNi-2Al catalysts in the methane combustion reaction exhibited a volcano-shaped curve as a function of Ni content, with a maximum being observed for the Pd/1.0Ni-2Al catalyst, which corresponded to the highest Pd2+ composition and reducibility.
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Pu ZY, Zhou H, Zheng YF, Huang WZ, Li XN, Appl. Surf. Sci., 410, 14 (2017)
Persson K, Ersson A, Jansson K, Iverlund N, Jaras S, J. Catal., 231(1), 139 (2005)
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Gao D, Zhang C, Wang S, Yuan Z, Wang S, Catal. Commun., 9, 2583 (2008)
Park JE, Kim BB, Park ED, Korean J. Chem. Eng., 32(11), 2212 (2015)
Yang W, Li D, Xu D, Wang X, J. Nat. Gas Chem., 18, 458 (2009)
Takeguchi T, Aoyama S, Ueda J, Kikuchi R, Eguchi K, Top. Catal., 23, 159 (2003)
Takeguchi T, Takeoh O, Aoyama S, Ueda J, Kikuchi R, Eguchi K, Appl. Catal. A: Gen., 252(1), 205 (2003)
Yin FX, Ji SF, Wu PY, Zhao FZ, Li CY, J. Catal., 257(1), 108 (2008)
Marti PE, Maciejewski M, Baiker A, Appl. Catal. B: Environ., 4(2-3), 225 (1994)
Guilhaume N, Primet M, J. Chem. Soc.-Faraday Trans., 90, 1541 (1994)
Liu Y, Wang S, Sun T, Gao D, Zhang C, Wang S, Appl. Catal. B: Environ., 119-120, 321 (2012)
Zou XL, Rui ZB, Song SQ, Ji HB, J. Catal., 338, 192 (2016)
Pan X, Zhang Y, Miao Z, Yang X, J. Energy Chem., 22, 610 (2013)
Widjaja H, Sekizawa K, Eguchi K, Arai H, Catal. Today, 47(1-4), 95 (1999)
Hoque MA, Kim K, Korean J. Chem. Eng., 31(8), 1316 (2014)
Burch R, Urbano FJ, Loader PK, Appl. Catal. A: Gen., 123(1), 173 (1995)
Boumaza A, Favaro L, Ledion J, Sattonnay G, Brubach J, Berthet P, Huntz A, Roy P, Tetot R, J. Solid State Chem., 182, 1171 (2009)
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Busca G, Catal. Today, 226, 2 (2014)
Rane S, Borg O, Yang J, Rytter E, Holmen A, Appl. Catal. A: Gen., 388(1-2), 160 (2010)
Rebours B, Caillerie JBDDL, Clause O, J. Am. Ceram. Soc., 116, 1707 (1994)
Zhang J, Xu HY, Jin XL, Ge QJ, Li WZ, Appl. Catal. A: Gen., 290(1-2), 87 (2005)
Vos B, Poels E, Bliek A, J. Catal., 198(1), 77 (2001)
Hong E, Sim HI, Shin CH, Chem. Eng. J., 292, 156 (2016)
Hong EP, Baek SW, Shin M, Suh YW, Shin CH, J. Ind. Eng. Chem., 54, 137 (2017)
Pyen S, Hong E, Shin M, Suh YW, Shin CH, Mol. Catal., 448, 71 (2018)
Arean CO, Mentruit MP, Lopez AL, Parra J, Colloids Surf. A: Physicochem. Eng. Asp., 180, 253 (2001)
Shen J, Hayes RE, Wu X, Semagina N, ACS Catal., 5, 2916 (2015)
Otto K, Haack L, Appl. Catal. B: Environ., 1, 1 (1992)
Mccarty JG, Catal. Today, 26(3-4), 283 (1995)
Borko L, Nagy I, Schay Z, Guczi L, Appl. Catal. A: Gen., 147(1), 95 (1996)
Muller CA, Maciejewski M, Koeppel RA, Baiker A, Catal. Today, 47(1-4), 245 (1999)
Castellazzi P, Groppi G, Forzatti P, Baylet A, Marecot P, Duprez D, Catal. Today, 155(1-2), 18 (2010)
Shi CK, Yang LF, Wang ZC, He XE, Cai JX, Li G, Wang XS, Appl. Catal. A: Gen., 243(2), 379 (2003)
