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Received August 15, 2018
Accepted October 10, 2018
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Adsorption and precipitation of anionic dye Reactive Red 120 from aqueous solution by aminopropyl functionalized magnesium phyllosilicate
Department of Biochemical and Polymer Engineering, Chosun University, 309 Pilmundaero, Dong-gu, Gwangju 61452, Korea 1Department of Environmental Engineering, Chosun University, 309 Pilmundaero, Dong-gu, Gwangju 61452, Korea
shinhj@chosun.ac.kr
Korean Journal of Chemical Engineering, January 2019, 36(1), 101-108(8), 10.1007/s11814-018-0168-8
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Abstract
Dye wastewater causing destruction in ecosystem from a variety of plants an operation needs various factors for environmental cleanup. To improve removal efficiency of dye wastewater, various adsorbents including clay and nonclay-related materials have been tried. The use of soluble aminopropyl functionalized magnesium phyllosilicate (Mg-AMP clay) as an adsorbent for the textile anionic dye Reactive Red 120 (RR 120) was examined thermodynamically and kinetically. The adsorption kinetics followed the pseudo-second-order and Langmuir isotherm equation fitted best models. A maximum amount of adsorption was determined to be 229.9mg/g, which is one of the highest values studied so far. An Mg-AMP clay dosage of 10mg/mL obtained from Langmuir model a maximum adsorption capacity of 229.94, 182.26 and 156.54mg/g at 298.15, 308.15 and 318.15 K, respectively. Moreover the thermodynamic activation parameters such as enthalpy and entropy were determined. We suggest the removal mechanism of RR 120 using Mg-AMP clay by adsorption and precipitation.
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Gong RM, Li M, Yang C, Sun YZ, Chen J, J. Hazard. Mater., 121(1-3), 247 (2005)
Brookstein DS, Dermatol. Clin., 27, 309 (2009)
Houk VS, Mutat. Res. Rev. Genet. Toxicol., 277, 91 (1992)
Crini G, Bioresour. Technol., 97(9), 1061 (2006)
Crini G, Badot PM, Prog. Polym. Sci, 33, 399 (2008)
Venkata RB, Sastray CA, Indian J. Environ. Prot., 7, 363 (1987)
Momenzadeh H, Tehrani-Bagha AR, Khosravi A, Gharanjig K, Holmberg K, Desalination, 271(1-3), 225 (2011)
Greluk M, Hubicki Z, Chem. Eng. Res. Des., 91(7), 1343 (2013)
Absalan G, Asadi M, Kamran S, Sheikhian L, Goltz DM, J. Hazard. Mater., 192(2), 476 (2011)
Xue YJ, Hou HB, Zhu SJ, Chem. Eng. J., 147(2-3), 272 (2009)
Abidi N, Errais E, Duplay J, Berez A, Jrad A, Schafer G, Ghazi M, Semhi K, Trabelsi-Ayadi M, J. Clean Prod., 86, 432 (2015)
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Babel S, Kurniawan TA, J. Hazard. Mater., 97(1-3), 219 (2003)
Patel HA, Somani RS, Bajaj HC, Jasra RV, Bull. Mat. Sci., 29, 133 (2006)
Okamoto M, Morita S, Taguchi H, Kim YH, Kotaka T, Tateyama H, Polymer, 41(10), 3887 (2000)
Patil AJ, Mann S, J. Mater. Chem., 18, 4605 (2008)
Melo MA, Oliveira FJBE, Airoldi C, Appl. Clay Sci., 42, 130 (2008)
Lee YC, Park WK, Yang JW, J. Hazard. Mater., 190(1-3), 652 (2011)
Han HK, Lee YC, Lee MY, Patil AJ, Shin HJ, ACS. Appl. Mater. Inter., 3, 2564 (2011)
Bui VKH, Park D, Lee YC, Chem. Eng. J., 336, 757 (2018)
Patil AJ, Muthusamy E, Mann S, Angew. Chem.-Int. Edit., 43, 4928 (2004)
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Langmuir I, J. Am. Chem. Soc., 38, 2221 (1916)
Freundlich HMF, J. Phys. Chem., 57, 385 (1906)
Abrams DS, Prausnitz JM, AIChE J., 21, 116 (1975)
Lagergren S, Handlingar, 24, 1 (1898)
Ho YS, McKay G, Process Biochem., 34(5), 451 (1999)
Lee YC, Kim EJ, Yang JW, Shin HJ, J. Hazard. Mater., 192(1), 62 (2011)
Lee YC, Park WK, Yang JW, J. Hazard. Mater., 190(1-3), 652 (2011)
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De Paiva LB, Morales AR, Diaz FRV, Appl. Clay Sci., 42, 8 (2008)
Demarchi CA, Campos M, Rodrigues CA, J. Environ. Chem. Eng., 1, 1350 (2013)
Chandrasekaran G, Han HK, Kim GJ, Shin HJ, Appl. Clay Sci., 53, 729 (2011)
Patil AJ, Li M, Mann S, Nanoscale, 5, 7161 (2013)
Viseras C, Cerezo P, Sanchez R, Salcedo I, Aguzzi C, Appl. Clay Sci., 48, 291 (2010)
Lee YC, Kim EJ, Shin HJ, Choi M, Yang JW, J. Ind. Eng. Chem., 18(3), 871 (2012)
Patil AJ, Muthusamy E, Seddon AM, Mann S, Adv. Mater., 15(21), 1816 (2003)
Patil AJ, Li M, Dujardin E, Mann S, Nano Lett., 7, 2660 (2007)
Burkett SL, Press A, Mann S, Chem. Mater., 9, 1071 (1997)
Mann S, Burkett SL, Davis SA, Fowler CE, Mendelson NH, Sims SD, Walsh D, Whilton NT, Chem. Mater., 9, 2300 (1997)
Lee YC, Kim JY, Shin HJ, Sep. Sci. Technol., 48(7), 1093 (2013)
Lee YC, Kim B, Farooq W, Chung J, Han JI, Shin HJ, Jeong SH, Park JY, Lee JS, Oh YK, Bioresour. Technol., 132, 440 (2013)
Farooq W, Lee YC, Han JI, Darpito CH, Choi M, Yang JW, Green Chem., 15, 749 (2013)
Nejib A, Joelle D, Fadhila A, Sophie G, Malika TA, Desalin. Water. Treat., 54, 1754 (2015)
Tabak A, Baltas N, Afsin B, Emirik M, Caglar B, Eren E, J. Chem. Technol. Biotechnol., 85(9), 1199 (2010)
