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Received March 17, 2019
Accepted May 21, 2019
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This is an Open-Access article distributed under the terms of the Creative Commons Attribution Non-Commercial License (http://creativecommons.org/licenses/bync/3.0) which permits
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Enhanced adsorption of Orange II on bagasse-derived biochar by direct addition of CTAB
1Department of Environmental and Municipal Engineering, North China University of Water Resources and Electric Power, Zhengzhou 450011, China 2Henan Key Laboratory of Water Environment Simulation and Treatment, North China University of Water Resources and Electric Power, Zhengzhou 450011, China 3School of Environmental Science and Engineering, Tianjin University, Tianjin 300072, China
Korean Journal of Chemical Engineering, August 2019, 36(8), 1274-1280(7), 10.1007/s11814-019-0304-0
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Abstract
Surface charge properties of an adsorbent always play an important role for the removal of contaminants from water. A cationic surfactant hexadecyl tri-methyl ammonium bromide (CTAB) was involved into adsorptive removal of Orange II (ORII) by bagasse biochars to realize an in-situ modification and an enhanced adsorption capability. Adsorption capacity of biochar (BC600) improved significantly from 1.66mg/g in the absence of CTAB to 4.42mg/g in the presence of 2.0mg/L CTAB. A more hydrophobic surface of bagasse biochar was favorable for the dye uptake in the presence of CTAB. Linear pseudo-second-order kinetic model fitted the kinetics data better at three pH conditions than pseudo-first-order kinetic model, whether in the presence and absence of CTAB. Both nonlinear pseudo-first-order and pseudo-second-order kinetic models were suitable to describe the experimental data. The maximal adsorption capacity in the absence of CTAB was very limited (41.4mg/g), while the adsorption isotherm curve in the presence of CTAB was almost linear, indicating a strong adsorption capability due to the introduction of CTAB. Direct addition of CTAB into wastewater is a potential technique for the enhanced removal of negatively-charged pollutants by bagasse biochar.
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