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Received February 14, 2019
Accepted June 1, 2019
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Competition of mixed divalent ions through supported liquid membranes: Co-ion and concentration effects on permeability
1Department of Chemical and Materials Engineering and Green Technology Research Center, Chang Gung University, Guishan District, Taoyuan 333, Taiwan 2Institute of Environmental Science, Engineering and Management, Industrial University of Ho Chi Minh City, Go Vap District, Ho Chi Minh City, Vietnam 3Department of Radiation Oncology, Chang Gung Memorial Hospital, Guishan District, Taoyuan 333, Taiwan
jessie@mail.cgu.edu.tw
Korean Journal of Chemical Engineering, August 2019, 36(8), 1328-1338(11), 10.1007/s11814-019-0322-y
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Abstract
Zn2+, Cu2+ and Ni2+ permeabilities through supported liquid membranes (SLMs) were determined experimentally from single, binary, and ternary ionic mixtures. Microporous polypropylene membrane was used as the frame to retain isopar-L solvent and di (2-ethylhexyl) phosphoric acid (D2EHPA) carrier. Sulfuric acid solution was used as a strip (receiving) solution. The ion permeability values were in the 10-7 - 10-6 cm2 s-1 range and increased with the concentrations of D2EHPA in isopar-L and the stripping sulfuric acid. The ion ideal selectivity ranged from 1.05 (Zn/Cu) to 8.40 (Zn/Ni), depending on the feed concentration. The single ion permeability was significantly higher than the binary mixtures, probably due to ion competition with D2EHPA carrier molecules. High selectivity was achieved using ternary mixtures: Zn2+ was the fast-permeating species due to preferential sorption with D2EHPA. Separating Zn2+ from Cu2+ and/or Ni2+ mixtures was most efficient with high D2EHPA concentration, concentrated H2SO4 strip solution, concentrated feed solution, and from multiple ionic mixes.
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References
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Parhi PK, J. Chem., 2013, 11 (2013)
Mai NL, Kim SH, Ha SH, Shin HS, Koo YM, Korean J. Chem. Eng., 30(9), 1804 (2013)
Yang XJ, Fane AG, Soldenhoff K, Ind. Eng. Chem. Res., 42(2), 392 (2003)
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Cooper CA, Lin YS, Gonzalez M, J. Membr. Sci., 229(1-2), 11 (2004)
Kemperman AJ, Bargeman D, Vandenboomgaard T, Strathmann H, Sep. Sci. Technol., 31(20), 2733 (1996)
Ho W, Podd TK, Environ. Prog. Sustainable Energy, 20, 44 (2001)
Bringas E, San Roman MF, Ortiz I, J. Chem. Technol. Biotechnol., 81(11), 1829 (2006)
Crabtree RH, Chem. Rev., 85, 245 (1985)
Sulaiman RNR, Othman N, J. Environ. Chem. Eng., 6, 1814 (2018)
Gherrou A, Kerdjoudj H, Molinari R, Drioli E, Sep. Purif. Technol., 28(3), 235 (2002)
Kunungo SB, Mohapatra R, J. Membr. Sci., 105(3), 227 (1995)
Sarangi K, Das RP, Hydrometallurgy, 71, 335 (2004)
Arous O, Gherrou A, Kerdjoudj H, Desalination, 161(3), 295 (2004)
Venkateswaran P, Gopalakrishnan AN, Palanivelu K, J. Environ. Sci., 19, 1446 (2007)
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He J, Li Y, Xue X, Ru H, Huang X, Yang H, RSC Adv., 5, 74961 (2015)
Nadimi H, Amirjani A, Fatmehsari DH, Firoozi S, Azadmehr A, Miner. Eng., 69, 177 (2014)
Surucu A, Eyupoglu V, Tutkun O, Desalination, 250(3), 1155 (2010)
Pereira DD, Rocha SDF, Mansur MB, Sep. Purif. Technol., 53(1), 89 (2007)
Bhatluri KK, Manna MS, Saha P, Ghoshal AK, J. Membr. Sci., 459, 256 (2014)
Nightingale ER, J. Phys. Chem., 63, 1381 (1959)
Gotfryd L, Pietek G, Physicochem. Probl. Miner. Process., 49, 133 (2013)
Group C, MCT Redbook: Solvent Extraction Reagents and Applications, Cognis Group, U.S.A. (2007).
Cheng CY, Hydrometallurgy, 56, 369 (2000)
Nikam G, Mahanwar K, Sabale S, Mohite B, Sep. Sci. Technol., 48(3), 493 (2013)
Nikam G, Mohite B, Res. J. Chem. Sci., 2, 75 (2012)
Mohammed AA, Hussein MA, Association of Arab Universities J. of Engineering Sciences, 25, 65 (2018).
Cole PM, Sole KC, Miner. Process. Extr. Metall. Rev., 24, 91 (2003)
Molinari R, Poerio T, Argurio P, J. Membr. Sci., 280(1-2), 470 (2006)
Belkhouche NE, Didi MA, Romero R, Jonsson JA, Villemin D, J. Membr. Sci., 284(1-2), 398 (2006)
Huang TC, Juang RS, J. Membr. Sci., 31, 209 (1987)
Molinari R, Argurio P, Poerio T, Sep. Purif. Technol., 70(2), 166 (2009)
Parhi P, Sarangi K, Mohanty SJM, Min., Metall. Explor., 29, 225 (2012)
Parhi PK, Sarangi K, Sep. Purif. Technol., 59(2), 169 (2008)
