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Received February 15, 2019
Accepted June 16, 2019
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Development of metal organic framework filled PDMS/PI composite membranes for biobutanol recovery
Yildiz Technical University, Chem. Eng. Dept., Davutpaşa, Istanbul, Turkey 1University of Santiago de Chile, Chem. Eng. Dept., Santiago, Chile
Korean Journal of Chemical Engineering, September 2019, 36(9), 1489-1498(10), 10.1007/s11814-019-0327-6
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Abstract
Butanol is a second generation biofuel with high potential to replace fossil fuels in the future. The main drawbacks in biobutanol production are the low yields of operation and high cost of separation. In this study, n-butanol recovery from its aqueous solutions was carried out by pervaporation as an alternative separation process using polyimide supported polydimethylsiloxane membranes, which were especially prepared for this purpose. To enhance the separation efficiency of the membrane, metal organic framework fillers of MOF-199 were included in its structure. Several combinations of polyimide supported PDMS active layered membranes were prepared with the fillers in each layer of the membrane, in both layers of membrane and membranes without fillers. Thus, the effect of the fillers on the separation performance was investigated. It was found that the inclusion of MOF-199 enhances the membrane performance; meanwhile, the support layer also contributes to mass transfer of n-butanol. Furthermore, the effect of the process parameters on the pervaporation performance was investigated. Results of pervaporation tests indicate that the developed membranes have a good potential for n-butanol recovery from aqueous mixtures.
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References
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Duan CJ, Jie XM, Liu DD, Cao YM, Yuan Q, J. Membr. Sci., 466, 92 (2014)
Yoon HC, Rallapalli PBS, Han SS, Beum HT, Jung TS, Cho DW, Ko M, Kim JN, Korean J. Chem. Eng., 32(12), 2501 (2015)
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Campbell J, Szekely G, Davies RP, Braddock DC, Livingston AG, J. Mater. Chem. A, 2, 9260 (2014)
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Brinda L, Rajan KS, Rayappan JBB, J. Appl. Sci., 12, 1778 (2012)
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Chae B, Hong DG, Jung YM, Won JC, Lee SW, Spectroc. Acta Pt. A-Molec. Biomolec. Spectr., 195, 1 (2018)
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Li YW, Yang RT, AIChE J., 54(1), 269 (2008)
Esmaielzadeh S, Ahmadizadegan H, Solid State Sci., 78, 46 (2018)
Huang CS, Sun RJ, Lu H, Yang Q, Hu J, Wang HL, Liu HL, Sep. Purif. Technol., 182, 110 (2017)
Ferreira P, Carvalho A, Correia TR, Antunes BP, Correia IJ, Alves P, Sci. Technol. Adv. Mater., 14, 1 (2013)
Kanungo M, Mettu S, Law KY, Daniel S, Langmuir, 30(25), 7358 (2014)
DeCoste JB, Peterson GW, Chem. Rev., 114(11), 5695 (2014)
DeCoste JB, Denny MS, Peterson GW, Mahle JJ, Cohen SM, Chem. Sci., 7, 2711 (2016)
Mukherjee S, Sharma S, Ghosh SK, APL Mater., 7, 050701 (2019)
Van Assche TRC, Duerinck T, Guttierez-Sevillano JJ, Calero S, Denayer JFM, San Francisco, CA, 13th AIChE Annual Meeting, November (2013).
Kusgens P, Rose M, Senkovska I, Fode H, Henschel A, Siegle S, Kaskel S, Microporous Mesoporous Mater., 120, 325 (2009)
Aminabhavi TM, Naidu BVK, Sridhar S, Rangarajan R, J. Appl. Polym. Sci., 95(5), 1143 (2005)
Koops GH, Nolten JA, Mulder MH, Smolders CA, J. Appl. Polym. Sci., 53(12), 1639 (1994)
Kanti P, Srigowri K, Madhuri J, Smitha B, Sridhar S, Sep. Purif. Technol., 40(3), 259 (2004)
Fouad EA, Feng XS, J. Membr. Sci., 323(2), 428 (2008)
Sun D, Yang P, Li L, Yang HH, Li BB, Korean J. Chem. Eng., 31(10), 1877 (2014)
Yeom CK, Dickson JM, Brook MA, Korean J. Chem. Eng., 13(5), 482 (1996)
