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Received April 18, 2020
Accepted July 7, 2020
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This is an Open-Access article distributed under the terms of the Creative Commons Attribution Non-Commercial License (http://creativecommons.org/licenses/bync/3.0) which permits
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Adsorption of Direct Red 23 dye from aqueous solution by means of modified montmorillonite nanoclay as a superadsorbent: Mechanism, kinetic and isotherm studies
1Environmental Science and Technology Research Center, Department of Environmental Health Engineering, School of Public Health, Shahid Sadoughi University of Medical Sciences, Yazd, Iran 2Student Research Committee, Shahid Sadoughi University of Medical Sciences, Yazd, Iran
arash.dalvand@gmail.com
Korean Journal of Chemical Engineering, December 2020, 37(12), 2192-2201(10), 10.1007/s11814-020-0629-8
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Abstract
A novel adsorbent of modified nanoclay was synthesized by covering of alum on the montmorillonite nanoclay (Al/nanoclay). Al/nanoclay was applied as an efficient superadsorbent to remove Direct Red 23 (DR23) from colored wastewater. The adsorbent was characterized by Fourier transform infrared spectroscopy, energy-dispersive Xray spectroscopy, and zeta potential analysis. The effects of various operating parameters, such as contact time, initial dye concentration, adsorbent dose, pH and ionic strength on the performance of adsorption, have been studied. The adsorption experiments showed that pH has an obvious effect on the adsorption efficiency and the highest percentage of DR23 dye removal was observed at pH 2. Zeta potential measurement confirmed that the adsorption mechanism is ascribed to electrostatic interaction between sulfonic groups of the anionic dye and the positive surface charge of the adsorbent. The pseudo-second-order kinetic model and the Langmuir isotherm were found to best describe the DR23 adsorption and the maximum monolayer adsorption capacity at the conditions of pH 2 and the adsorbent dose of 0.05 g/L was 2,500mg/g. The findings recommend that Al/nanoclay can be successfully used for DR23 dye removal from the colored wastewater.
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Liu N, Wang H, Weng CH, Hwang CC, Arabian J. Chem., 11, 1281 (2018)
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Lucilha AC, Bonancea CE, Barreto WJ, Takashima K, Spectroc. Acta Pt. A-Molec. Biomolec. Spectr., 75, 389 (2010)
Paz A, Carballo J, Perez MJ, Dominguez JM, Chemosphere, 181, 168 (2017)
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Mollah MYA, Gomes JAG, Das KK, Cocke DL, J. Hazard. Mater., 174(1-3), 851 (2010)
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Dias NC, Bassin JP, Sant’Anna GL, Dezotti M, Int. Biodeterior. Biodegrad., 144, 104742 (2019)
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Pormazar SM, Dalvand A, Int. J. Environ. Anal. Chem., 1 (2020)
Nawaz MS, Ahsan M, Alex. Eng. J., 53, 717 (2014)
Cheruiyot GK, Wanyonyi WC, Kiplimo JJ, Maina EN, Sci. Afr., 5, e00116 (2019)
Salehi R, Dadashian F, Ekrami E, Prog. Color Colorants Coat., 11, 9 (2018)
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Alver E, Metin AU, Chem. Eng. J., 200, 59 (2012)
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Almasri DA, Rhadfi T, Atieh MA, Mckay G, Ahzi S, Chem. Eng. J., 335, 1 (2018)
Chang J, Ma J, Ma Q, Zhang D, Qiao N, Hu M, Ma H, Appl. Clay Sci., 119, 132 (2016)
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Zhu Z, Ouyang S, Li P, Shan L, Ma R, Zhang P, Appl. Clay Sci., 188, 105500 (2020)
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Banerjee S, Chattopadhyaya MC, Arabian J. Chem., 10, S1629 (2017)
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Abbasi H, Asgari H, Global Nest J., 20, 582 (2018)
Inyinbor AA, Adekola FA, Olatunji GA, Water Resour. Ind., 15, 14 (2016)
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Konicki W, Aleksandrzak M, Moszynski D, Mijowska E, J. Colloid Interface Sci., 496, 188 (2017)
Fathi MR, Asfaram A, Farhangi A, Spectroc. Acta Pt. A-Molec. Biomolec. Spectr., 135, 364 (2015)
Chang PH, Li Z, Jean JS, Jiang WT, Wang CJ, Lin KH, Appl. Clay Sci., 67, 158 (2012)
Kim MH, Hwang CH, Bin Kang S, Kim S, Park SW, Yun YS, Won SW, Chem. Eng. J., 280, 18 (2015)
Mouni L, Belkhiri L, Bollinger JC, Bouzaza A, Assadi A, Tirri A, Dahmoune F, Madani K, Remini H, Appl. Clay Sci., 153, 38 (2018)
Zhu HY, Jiang R, Xiao L, Appl. Clay Sci., 48, 522 (2010)
Fideles RA, Ferreira GMD, Teodoro FS, Adarme OFH, da Silva LHM, Gil LF, Gurgel LVA, J. Colloid Interface Sci., 515, 172 (2018)
Harrache Z, Abbas M, Aksil T, Trari M, Microchem. J., 144, 180 (2019)
Deniz F, Karaman S, Microchem. J., 99, 296 (2011)
Hassan AF, Abdel-Mohsen AM, Fouda MMG, Carbohydr. Polym., 102, 192 (2014)
Elhadj M, Samira A, Mohamed T, Djawad F, Asma A, Djamel N, Sep. Sci. Technol., 55(5), 867 (2020)
Bhatti HN, Jabeen A, Iqbal M, Noreen S, Naseem Z, J. Mol. Liq., 237, 322 (2017)
Maneerung T, Liew J, Dai YJ, Kawi S, Chong C, Wang CH, Bioresour. Technol., 200, 350 (2016)
Shin HS, Kim JH, Process Biochem., 51(7), 917 (2016)
Li C, Xia H, Zhang L, Peng J, Cheng S, Shu J, Zhang S, Res. Chem. Intermed., 44, 2231 (2018)
Bayramoglu G, Yilmaz M, Fiber Polym., 19, 877 (2018)
Othman NH, Alias NH, Shahruddin MZ, Bakar NFA, Him NRN, Lau WJ, J. Environ. Chem. Eng., 6, 2803 (2018)
de Sousa DNR, Insa S, Mozeto AA, Petrovic M, Chaves TF, Fadini PS, Chemosphere, 205, 137 (2018)
Konicki W, Pelech I, Mijowska E, Jasinska I, Chem. Eng. J., 210, 87 (2012)
Kasperiski FM, Lima EC, dos Reis GS, da Costa JB, Dotto GL, Dias SLP, Cunha MR, Pavan FA, Correa CS, Chem. Eng. Commun., 205(10), 1520 (2018)
Mahmoodi NM, Taghizadeh A, Taghizadeh M, Baglou MAS, J. Environ. Chem. Eng., 7, 103243 (2019)
Puri C, Sumana G, Appl. Clay Sci., 166, 102 (2018)
Luo ZX, Gao ML, Ye YG, Yang SF, Appl. Surf. Sci., 324, 807 (2015)
Yin J, Pei M, He Y, Du Y, Guo W, Wang L, RSC Adv., 5, 89839 (2015)
Hosseinzadeh H, Zoroufi S, Mahdavinia GR, Polym. Bull., 72(6), 1339 (2015)
Bhattacharyya R, Ray SK, Chem. Eng. J., 260, 269 (2015)
Olad A, Azhar FF, Fiber Polym., 15, 1321 (2014)
Fan H, Zhou L, Jiang X, Huang Q, Lang W, Appl. Clay Sci., 95, 150 (2014)
Shi YR, Xue ZH, Wang XM, Wang L, Wang AQ, Polym. Bull., 70(4), 1163 (2013)
