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- In relation to this article, we declare that there is no conflict of interest.
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Received October 27, 2019
Accepted January 12, 2020
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This is an Open-Access article distributed under the terms of the Creative Commons Attribution Non-Commercial License (http://creativecommons.org/licenses/bync/3.0) which permits
unrestricted non-commercial use, distribution, and reproduction in any medium, provided the original work is properly cited.
Copyright © KIChE. All rights reserved.
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Removal of U(VI) from aqueous solution using carboxymethyl cellulose-modified Ca-rectorite hybrid composites
1Center for Environment and Water Resource, College of Chemistry and Chemical Engineering, Central South University, Changsha 410083, P. R. China 2School of Resources & Environmental Engineering, Hefei University of Technology, Hefei 230009, Anhui, P. R. China 3State Key Laboratory of Lake Science and Environment, Nanjing Institute of Geography and Limnology, Chinese Academy of Sciences, Nanjing 210008, China 4Jiangsu Key Laboratory of Chemical Pollution Control and Resources Reuse, School of Environmental and Biological Engineering, Nanjing University of Science and Technology, Nanjing 210094, P. R. China
shuheng.hu@163.com
Korean Journal of Chemical Engineering, May 2020, 37(5), 776-783(8), 10.1007/s11814-020-0492-7
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Abstract
Uranium (VI), as a toxic contaminant, is a potential detriment to human health and environmental safety. In this experiment, carboxymethyl cellulose/Ca-rectorite composite material (Ca-REC/CMC) was prepared by crosslinking reaction to remove U(VI) from the liquid. The crystal structure was detected by X-ray diffraction (XRD) and surface structure and morphology of the materials were investigated by scanning electron microscopy (SEM). The surface functional groups of prepared materials were detected by Fourier transform infrared spectroscopy (FT-IR). The adsorption capacity of Ca-REC/CMC improved obviously after being modified by CMC. The adsorption capacity of Ca-REC/CMC was closely related to ionic strength and pH. According to thermodynamic parameter calculation, the adsorption process was endothermic and spontaneous. Adsorption isotherms could be depicted perfectly by the Langmuir model. Ca-REC/CMC maintained stability and regeneration after recycling six times. The adsorption mechanism, including electrostatic interactions and ionic interaction, was investigated by the X-ray photoelectron spectroscopy (XPS). Ca-REC/CMC is considered as remarkable potential material for removing U(VI) from the water environment.
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