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Received January 4, 2020
Accepted February 27, 2020
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This is an Open-Access article distributed under the terms of the Creative Commons Attribution Non-Commercial License (http://creativecommons.org/licenses/bync/3.0) which permits
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Highly efficient removal from aqueous solution by adsorption of Maxilon Red GRL dye using activated pine sawdust
Department of Environmental Engineering, Engineering Faculty, Sivas Cumhuriyet University, Sivas, 58140, Turkey 1Department of Environmental Engineering, Graduate School of Sciences, Sivas Cumhuriyet University, Sivas, 58140, Turkey
Korean Journal of Chemical Engineering, June 2020, 37(6), 985-999(15), 10.1007/s11814-020-0526-1
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Abstract
Pine sawdust, to which sulfuric acid was applied (APSD), was utilized as an inexpensive adsorbent to perform the batch adsorptive removal from a synthetic dye solution of Maxilon Red GRL (MR GRL). The activated adsorbent was characterized by the points of zero charge, FTIR, N2 adsorption-desorption, SEM, and SEM-EDX analyses. According to the removal results, the highest efficiency of the dye adsorption was reached at 180min. MR GRL removal of 99.35% was achieved using APSD under the optimum conditions (pH=5.7-6.0, temperature=298 K, dye concentration= 250mg/L, and adsorbent dosage=8 g/L). The Langmuir isotherm represents the best explanation model for the experimental data, which has the highest adsorption capacity of 312.5mg/g at 318 K. The compatibility of adsorption with the Langmuir isotherm showed that adsorption was reversible and physical. The other results obtained confirmed this situation. The kinetic research demonstrated that the sorption process was realized in accordance with the pseudo-second- order kinetic model. The thermodynamic parameters revealed that the MR GRL adsorption occurred spontaneously and was exothermic. The findings of the present research confirm that acid-activated pine sawdust may be utilized to remove MR GRL dye from aqueous solutions as a low-cost and efficient adsorbent.
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Dogan M, Karaoglu MH, Alkan M, J. Hazard. Mater., 165(1-3), 1142 (2009)
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El-Sayed G, Int. Res. J. Pure Appl. Chem., 4, 402 (2014)
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Karaoglu MH, Dogan M, Alkan M, Microporous Mesoporous Mater., 122, 20 (2009)
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Mehrabi F, Vafaei A, Ghaedi M, Ghaedi AM, Alipanahpour Dil E, Asfaram A, Ultrason. Sonochem., 38, 672 (2017)
Salleh MAM, Mahmoud DK, Karim WAWA, Idris A, Desalination, 280(1-3), 1 (2011)
Jain SN, Gogate PR, J. Mol. Liq., 243, 132 (2017)
Deniz F, Kepekci RA, Microchem. J., 132, 172 (2017)
Yakout SM, Hassan MR, El-Zaidy ME, Shair OH, Salih AM, 14(2), 4560 (2019).
Dulman V, Cucu-Man SM, J. Hazard. Mater., 162(2-3), 1457 (2009)
Ozacar M, Sengil IA, Bioresour. Technol., 96(7), 791 (2005)
Batzias FA, Sidiras DK, J. Hazard. Mater., 114(1-3), 167 (2004)
Garg VK, Gupta R, Yadav AB, Kumar R, Bioresour. Technol., 89(2), 121 (2003)
Ofomaja AE, Chem. Eng. J., 143(1-3), 85 (2008)
Akhouairi S, Ouachtak H, Addi AA, Jada A, Douch J, Water. Air. Soil Pollut., 230, 181 (2019)
Ferrero F, J. Hazard. Mater., 142(1-2), 144 (2007)
Hamdaoui O, J. Hazard. Mater., 135(1-3), 264 (2006)
Salazar-Rabago JJ, Leyva-Ramos R, Rivera-Utrilla J, Ocampo-Perez R, Cerino-Cordova FJ, Sustain. Environ. Res., 27, 32 (2017)
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Ferro-Garcia MA, Rivera-Utrilla J, Bautista-Toledo I, Moreno-Castilla C, Langmuir, 14(7), 1880 (1998)
Kusmierek K, Swiatkowski A, Pol. J. Chem. Technol., 17, 23 (2015)
Trinh TK, Kang LS, Environ. Eng. Res., 15, 63 (2010)
Foo KY, Hameed BH, Bioresour. Technol., 111, 425 (2012)
Gul K, Sohni S, Waqar M, Ahmad F, Norulaini NAN, Omar AKM, Carbohydr. Polym., 152, 520 (2016)
Babic BM, Milonjic SK, Polovina MJ, Kaludierovic BV, Carbon, 37, 477 (1999)
Movasaghi Z, Yan B, Niu C, Ind. Crop. Prod., 127, 237 (2019)
Sidiras D, Batzias F, Schroeder E, Ranjan R, Tsapatsis M, Chem. Eng. J., 171(3), 883 (2011)
Lykiema J, Sing KSW, Haber J, Kerker M, Wolfram E, et al., Pure Appl. Chem., 57, 603 (1985)
Ma A, Mm M, J. Chromatogr. Sep. Technol., 7, 1 (2016)
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Yang P, Xu Y, Tuo J, Li A, Liu L, Shi H, R. Soc. Open Sci., 6, 181986 (2019)
Lafi R, Hafiane A, J. Taiwan Inst. Chem. Eng., 58, 424 (2016)
Deniz F, Kepekci RA, J. Mol. Liq., 219, 194 (2016)
El-Said AG, J. Am. Sci., 6, 143 (2010)
Wan Ngah WS, Hanafiah MAKM, BioChemEng. J., 39, 521 (2008)
Moussavi G, Barikbin B, Chem. Eng. J., 162(3), 893 (2010)
Chai XL, Zhao YC, J. Hazard. Mater., 137(1), 410 (2006)
Kuleyin A, Aydin F, Environ. Prog. Sustain. Energy, 30, 141 (2011)
Akpomie KG, Dawodu FA, Adebowale KO, Alexandria Eng. J., 54(3), 757 (2015)
Nadavala SK, Swayampakula K, Boddu VM, Abburi K, J. Hazard. Mater., 162(1), 482 (2009)
Tan IAW, Ahmad AL, Hameed BH, J. Hazard. Mater., 154(1-3), 337 (2008)
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Ali N, Pal P, Banat F, Srinivasakannan C, Sep. Sci. Technol., 54(16), 2671 (2019)
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Dada AO, Olalekan AP, Olatunya AM, Dada O, IOSR J. Appl. Chem., 3, 38 (2012)
Foo KY, Hameed BH, Chem. Eng. J., 156(1), 2 (2010)
Murthy TPK, Gowrishankar BS, Prabha MNC, Kruthi M, Krishna RH, Microchem. J., 146, 192 (2019)
Reed BE, Matsumoto MR, Sep. Sci. Technol., 28, 2179 (1993)
Akalin HA, Hicsonmez U, Yılmaz H, J. Turk. Chem. Soc. Sect. Chem., 5(1), 85 (2018)
Ayawei N, Ebelegi AN, Wankasi D, J. Chem., 2017, 1 (2017)
Gao Y, Li Y, Zhang L, Huang H, Hu JJ, Shah SM, Su XG, J. Colloid Interface Sci., 368, 540 (2012)
Kumar KV, Sivanesan S, Dyes Pigment., 72, 124 (2007)
Rezania H, Vatanpour V, Salehi E, Gavari N, Shockravi A, Ehsani M, J. Polym. Environ., 27, 1790 (2019)
Ciner F, Glob. NEST J., 20, 1 (2017)
Cebeci MS, Askal M, Glob. NEST J., 20, 25 (2017)
Irinislimane H, Belhaneche-Bensemra N, Chem. Eng. Commun., 204(8), 897 (2017)
Koyuncu M, Orient. J. Chem., 25(1), 35 (2009)
Koyuncu M, Asian J. Chem., 21, 5458 (2009)
Aljeboree AM, Alshirifi AN, Alkaim AF, Arab. J. Chem., 10, 3381 (2017)
Witek-Krowiak A, Chem. Eng. J., 171(3), 976 (2011)
Alkan M, Demirbas O, Celikcapa S, Dogan M, J. Hazard. Mater., 116(1-2), 135 (2004)
Gupta N, Kushwaha AK, Chattopadhyaya MC, Arab. J. Chem., 9, 707 (2016)
Khan MA, Othman ZAA, Kumar M, Ola MS, Siddique MR, Desalination Water Treat., 56, 146 (2015)
Gong R, Sun Y, Chen J, Liu H, Yang C, Dyes Pigment., 67, 175 (2005)
El Boujaady H, Mourabet M, El Rhilassi A, Bennani-Ziatni M, El Hamri R, Taitai A, J. Saudi Chem. Soc., 21, 94 (2017)
