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Received February 3, 2020
Accepted August 2, 2020
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This is an Open-Access article distributed under the terms of the Creative Commons Attribution Non-Commercial License (http://creativecommons.org/licenses/bync/3.0) which permits
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Effect of halloysite nanotubes incorporation on morphology and CO2/CH4 separation performance of Pebax-based membranes
Center of Excellence for Membrane Science and Technology, School of Chemical, Petroleum and Gas Engineering, Iran University of Science and Technology (IUST), Narmak, Tehran, Iran
torajmohammadi@iust.ac.ir
Korean Journal of Chemical Engineering, January 2021, 38(1), 104-113(10), 10.1007/s11814-020-0650-y
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Abstract
Mixed-matrix gas separation membranes were prepared by embedding various content of halloysite nanotubes (HNTs) (0, 0.5, 1, 1.5, and 2 wt%) within poly (ether-block-amide) matrix. XRD, FT-IR, TGA, and SEM analyses were conducted to study crystal structure, chemical bonds changes, thermal resistance, and cross-sectional morphology of the resultant membranes, respectively. Permeability values of pure CH4 and CO2 gases through the synthesized neat and mixed-matrix membranes (MMMs) were experimentally determined at constant temperature (25 °C) and several pressures (4, 6, 8, and 10 bar). The obtained results exhibited improved CO2 permeability of the MMMs comparing with the pristine Pebax membrane. As an example, at a pressure of 4 bar, raising the incorporated HNTs loading from 0 to 2wt% enhanced the permeability of CO2 from 76.50 to 101.23 Barrer.
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Rahman MM, Filiz V, Shishatskiy S, Abetz C, Neumann S, Bolmer S, Khan MM, Abetz V, J. Membr. Sci., 437, 286 (2013)
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Aghaei Z, Naji L, Asl VH, Khanbabaei G, Dezhagah F, Sep. Purif. Technol., 199, 47 (2018)
Dorosti F, Alizadehdakhel A, Chem. Eng. Res. Des., 136, 119 (2018)
Li T, Pan YC, Peinemann KV, Lai ZP, J. Membr. Sci., 425, 235 (2013)
Azizi N, Mohammadi T, Behbahani RM, J. Nat. Gas Sci. Eng., 37, 39 (2017)
Baker R, Membrane technology and applications, Wiley, Newark, California, USA (2012).
Bondar VI, Freeman BD, Pinnau I, J. Polym. Sci. B: Polym. Phys., 38(15), 2051 (2000)
Azizi N, Mahdavi HR, Isanejad M, Mohammadi T, J. Polym. Res., 24, 141 (2017)
Wang M, Wang Z, Zhao S, Wang JX, Wang SC, Chin. J. Chem. Eng., 25(11), 1581 (2017)
George G, Bhoria N, AlHallaq S, Abdala A, Mittal V, Sep. Purif. Technol., 158, 333 (2016)
Ren X, Ren J, Li H, Feng S, Deng M, Int. J. Greenh. Gas Control, 8, 111 (2012)
Zhao L, Chen YX, Wang B, Sun CH, Chakraborty S, Ramasubramanian K, Dutta PK, Ho WSW, J. Membr. Sci., 498, 1 (2016)
Chen YX, Wang B, Zhao L, Dutta P, Ho WSW, J. Membr. Sci., 495, 415 (2015)
Di Lorenzo ML, Pyda M, Wunderlich B, J. Polym. Sci. B: Polym. Phys., 39(14), 1594 (2001)
Hatfield GR, Guo Y, Killinger WE, Andrejak RA, Roubicek PM, Macromolecules, 26, 6350 (1993)
Konyukhova EV, Buzin AI, Godovsky YK, Thermochim. Acta, 391(1-2), 271 (2002)
Azizi N, Mohammadi T, Behbahani RM, J. Energy Chem., 26, 454 (2017)
Robeson LM, J. Membr. Sci., 62, 165 (1991)
Robeson LM, J. Membr. Sci., 320(1-2), 390 (2008)
Feng SC, Ren JZ, Hua KS, Li H, Ren XL, Deng MC, Sep. Purif. Technol., 116, 25 (2013)
Karthikeyan CS, Nunes SP, Prado LASA, Ponce ML, Silva H, Ruffmann B, Schulte K, J. Membr. Sci., 254(1-2), 139 (2005)
Wang L, Li Y, Li S, Ji P, Jiang C, J. Energy Chem., 23, 717 (2014)
Khoshkharam A, Azizi N, Behbahani RM, Ghayyem MA, Pet. Sci. Technol., 35, 667 (2017)
Dai Y, Ruan XH, Yan ZJ, Yang K, Yu M, Li H, Zhao W, He GH, Sep. Purif. Technol., 166, 171 (2016)
Jomekian A, Behbahani RM, Mohammadi T, Kargari A, J. Nat. Gas Sci. Eng., 31, 562 (2016)
Ignacio LE, Ant L, Karl S, Emilio B, Open J. Polym. Chem., 2012, 63 (2012)
Azizi N, Arzani M, Mahdavi HR, Mohammadi T, Korean J. Chem. Eng., 34(9), 2459 (2017)
Azizi N, Isanejad M, Mohammadi T, Behbahani RM, Front Chem. Sci. Eng., 13, 517 (2019)
Xu LW, Xiang L, Wang CQ, Yu J, Zhang LX, Pan YC, Chin. J. Chem. Eng., 25(7), 882 (2017)
Zhao D, Ren J, Li H, Hua K, Deng M, J. Energy Chem., 23, 227 (2014)
Zhao D, Ren JZ, Li H, Li XX, Deng MC, J. Membr. Sci., 467, 41 (2014)
Jazebizadeh MH, Khazraei S, Silicon, 9, 775 (2017)
Murali RS, Ismail AF, Rahman MA, Sridhar S, Sep. Purif. Technol., 129, 1 (2014)
Nafisi V, Hagg MB, J. Membr. Sci., 459, 244 (2014)
Ehsani A, Pakizeh M, J. Taiwan Inst. Chem. Eng., 66, 414 (2016)
Murali RS, Padaki M, Matsuura T, Abdullah MS, Ismail AF, Sep. Purif. Technol., 132, 187 (2014)
Ismail AF, Hashemifard SA, Matsuura T, J. Membr. Sci., 379(1-2), 378 (2011)
Hashemifard SA, Ismail AF, Matsuura T, J. Colloid Interface Sci., 359(2), 359 (2011)
Azizi N, Mohanunadi T, Behbahani RM, Chem. Eng. Res. Des., 117, 177 (2017)
Isanejad M, Azizi N, Mohammadi T, J. Appl. Polym. Sci., 134, 44531 (2017)
Xiang L, Pan YC, Zeng GF, Jiang JL, Chen J, Wang CQ, J. Membr. Sci., 500, 66 (2016)
Fan TT, Xie WL, Ji XY, Liu C, Feng X, Lu XH, Chin. J. Chem. Eng., 24(11), 1513 (2016)
Wang SF, Liu Y, Huang SX, Wu H, Li YF, Tian ZZ, Jiang ZY, J. Membr. Sci., 460, 62 (2014)
Stern S, J. Polym. Sci. Part A.2: Polym. Phys., 6, 1933 (1968).
Kim JH, Lee YM, J. Membr. Sci., 19, 209 (2001)
Farashi Z, Azizi N, Homayoon R, Pet. Sci. Technol., 37, 2412 (2019)
Ismail AF, Khulbe KC, Matsuura T, Gas separation membranes, Springer, Switzerland (2015).
Wang YB, Ren JZ, Deng MC, Sep. Purif. Technol., 77(1), 46 (2011)
Murali RS, Sridhar S, Sankarshana T, Ravikumar YVL, Ind. Eng. Chem. Res., 49(14), 6530 (2010)
Yampolskii Y, Freeman B, Membrane gas separation, Wiley Online Library (2010).
Ghadimi A, Amirilargani M, Mohammadi T, Kasiri N, Sadatnia B, J. Membr. Sci., 458, 14 (2014)
Ariazadeh M, Farashi Z, Azizi N, Khajouei M, Korean J. Chem. Eng., 37(2), 295 (2020)
Murali RS, Ismail AF, Rahman MA, Sridhar S, Sep. Purif. Technol., 129, 1 (2014)
Rabiee H, Alsadat SM, Soltanieh M, Mousavi SA, Ghadimi A, J. Ind. Eng. Chem., 27, 223 (2015)
Sharifloo MM, Ghaee A, Salimi E, Sadatnia B, Mansourpour Z, Int. J. Polymer. Mater. Polymer. Biomater., 68, 762 (2019)
Yu B, Cong HL, Li ZJ, Tang JG, Zhao XS, J. Appl. Polym. Sci., 130(4), 2867 (2013)
Nordin NAHM, Racha SM, Matsuura T, Misdan N, Sani NAA, Ismail AF, Mustafa A, RSC Adv., 5, 43110 (2015)
Nordin NAHM, Ismail AF, Mustafa A, Murali RS, Matsuura T, RSC Adv., 5, 30206 (2015)
Dorosti F, Omidkhah M, Abedini R, J. Nat. Gas Sci. Eng., 25, 88 (2015)
Meshkat S, Kaliaguine S, Rodrigue D, Sep. Purif. Technol., 200, 177 (2018)
Ghadimi A, Mohammadi T, Kasiri N, Int. J. Hydrog. Energy, 40(31), 9723 (2015)
Farashi Z, Azizi S, Arzhandi MRD, Noroozi Z, Azizi N, J. Nat. Gas Sci. Eng., 72, 103019 (2019)
Sadeghi M, Talakesh MM, Ghalei B, Shafiei M, J. Membr. Sci., 427, 21 (2013)
Rahman MM, Filiz V, Shishatskiy S, Abetz C, Neumann S, Bolmer S, Khan MM, Abetz V, J. Membr. Sci., 437, 286 (2013)
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Aghaei Z, Naji L, Asl VH, Khanbabaei G, Dezhagah F, Sep. Purif. Technol., 199, 47 (2018)
Dorosti F, Alizadehdakhel A, Chem. Eng. Res. Des., 136, 119 (2018)
Li T, Pan YC, Peinemann KV, Lai ZP, J. Membr. Sci., 425, 235 (2013)
