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Received March 24, 2021
Accepted May 20, 2021
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This is an Open-Access article distributed under the terms of the Creative Commons Attribution Non-Commercial License (http://creativecommons.org/licenses/bync/3.0) which permits
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Fabrication and modification of cellulose aerogels from Vietnamese water hyacinth for oil adsorption application
La Nam Phat1 2
Tran Quoc Thang3
Huynh Cam Nguyen1 2
Dang Thi My Duyen1 2
Dao Xuan Tien3
Bui Dang Dang Khoa1 2
Pham Tan Khang1 2
Nguyen Thi Huong Giang1 2
Hoang Minh Nam1 2
Mai Thanh Phong1 2
Nguyen Huu Hieu1 2†
1VNU-HCM, Key Laboratory of Chemical Engineering and Petroleum Processing (Key CEPP Lab), Ho Chi Minh City University of Technology (HCMUT), 268 Ly Thuong Kiet Street, District 10, Ho Chi Minh City, Vietnam 2Faculty of Chemical Engineering, Ho Chi Minh City University of Technology (HCMUT), 268 Ly Thuong Kiet Street, District 10, Ho Chi Minh City, Vietnam 3Faculty of Chemistry Ho Chi Minh City University of Science (HCMUS), 227 Nguyen Van Cu Street, District 5, Ho Chi Minh City, Vietnam
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Korean Journal of Chemical Engineering, November 2021, 38(11), 2247-2255(9), 10.1007/s11814-021-0853-x
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Abstract
Recycling biomass to cellulose aerogel (Cell-A) provides a promising approach to develop adsorbent materials for spilled-oil recovery. In this work, Cell-A was fabricated from Vietnamese water hyacinth via crosslinking methods using PVA as a crosslinker and freeze-drying process. Various cellulose to PVA ratios were investigated to obtain the optimal synthesis condition. The Cell-A was additionally modified by dip-coating in poly(dimethylsiloxane) (PDMS) and pyrolyzing to form PDMS-coated cellulose aerogels (Cell-AP) and carbon aerogels (CA), respectively. Results of the oil adsorption tests show that pyrolysis produced aerogels with greater adsorption capacity with an optimal mass ratio of 15 : 1 cellulose to PVA. Furthermore, the pseudo-second-order model was found to be more accurate than the pseudo-first-order model for the study of oil absorption kinetics. As a result, the modified cellulose aerogel is promising for replacing earth-unfriendly polymer-based oil sorbents due to their high oil absorption capacity.
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Vargas AMM, Cazetta AL, Kunita MH, Silva TL, Almeida VC, Chem. Eng. J., 168(2), 722 (2011)
