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Received August 25, 2020
Accepted October 3, 2020
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Recent advances in the synthesis of mesoporous materials and their application to lithium-ion batteries and hybrid supercapacitors

Chemical & Process Technology Division, Korea Research Institute of Chemical Technology (KRICT), 141 Gajeongro, Daejeon 34114, Korea 1Energy & Environment Division, Korea Institute of Ceramic Engineering and Technology (KICET), Jinju, Gyeongnam 52851, Korea 2School of Chemical Engineering & Materials Science, Chung-Ang University (CAU), 84 Heukseok-ro, Dongjak-gu, Seoul 06974, Korea 3Department of Chemical Engineering, Ajou University, Worldcupro 206, Suwon 16499, Korea
changshin@cau.ac.kr
Korean Journal of Chemical Engineering, February 2021, 38(2), 227-247(21), 10.1007/s11814-020-0693-0
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Abstract

The ever-growing demand for high performance energy storage systems has fueled the development of advanced electrode materials with light weight, high energy/power densities, and stable cycle life. Mesoporous materials play an important role in achieving these goals because of their unique features such as high surface area, tunable pore size, pore volume, and pore structures, as well as adjustable particle size and morphology. In this review, we summarize the recent progress in the synthesis of mesoporous materials and their applications in lithium-ion batteries (LIBs) and lithium-ion hybrid supercapacitors (Li-HSCs) over the past ten years. The block copolymer guided softtemplate route is highlighted as a simple and versatile tool for designing mesoporous materials with controlled nanoand macrostructures without complicated synthetic procedures. The structural/morphological benefits of designed mesoporous materials translate into highly improved electrochemical performance in LIBs and Li-HSCs. Finally, future challenges and perspectives on the development of mesoporous materials in energy storage devices are provided, which will be useful both in academia and in industry.

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