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Received July 22, 2020
Accepted October 17, 2020
- This is an Open-Access article distributed under the terms of the Creative Commons Attribution Non-Commercial License (http://creativecommons.org/licenses/bync/3.0) which permits unrestricted non-commercial use, distribution, and reproduction in any medium, provided the original work is properly cited.
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Removal efficiency optimization of Pb2+ in a nanofiltration process by MLP-ANN and RSM
Department of Chemical Engineering, University of Science and Technology of Mazandaran, Behshahr, Iran
m_r_emami@mazust.ac.ir
Korean Journal of Chemical Engineering, February 2021, 38(2), 316-325(10), 10.1007/s11814-020-0698-8
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Abstract
Using computational intelligence for prediction, modeling, and optimization of chemical process behavior could save costs and time. This study’s main goal was to predict and optimize removal efficiency and permeate flux behavior of Pb2+ aqueous solution in a nanofiltration process through using response surface methodology (RSM) and multilayer perceptron (MLP) neural network. A regression coefficient R2=0.99 was obtained for both removal efficiency and permeate flux in the RSM model. Also, the F-value for the removal efficiency and permeate flux was 394.79 and 1888.85, respectively. Different MLP structures for predicting removal efficiency and permeate flux behavior of lead ion in aqueous solutions were investigated. The best structure was obtained for two hidden layers with nine (tansig transfer function) and three (logsig transfer function) neurons. The values of R=0.9993, R2=0.9986, MSE=0.402 and MAE= 0.409 for the best structure were obtained. Finally, the the removal efficiency was optimized through RSM based on the experimental data. It was concluded that optimum mode selected for membrane composition of PSF=10.04%, NMP= 88.98%, and PAN-CMC-41=0.98% (wt%) 53.17 ppm as lead ion concentration in solution and 30.31 min for filtration time achieved the maximum value of removal efficiency equal to 90.68%.
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References
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Tang SY, Qiu TR, Korean J. Chem. Eng., 36(8), 1321 (2019)
Hosseini SM, Karami F, Farahani SK, Bandehali S, Shen J, Bagheripour E, Seidypoor A, Korean J. Chem. Eng., 37(5), 866 (2020)
Goel V, Mandal UK, Korean J. Chem. Eng., 36(4), 573 (2019)
Nabian N, Ghoreyshi AA, Rahimpour A, Shakeri M, Korean J. Chem. Eng., 32(11), 2204 (2015)
Arif Z, Sethy NK, Kumari L, Mishra PK, Verma B, Korean J. Chem. Eng., 36(7), 1148 (2019)
Yousefi N, Nabizadeh R, Nasseri S, Khoobi M, Nazmara S, Mahvi AH, Korean J. Chem. Eng., 34(8), 2342 (2017)
Alawady AR, Alshahrani AA, Aouak TA, Alandis NM, Chem. Eng. J., 388, 124267 (2020)
Modi A, Bellare J, J. Water Process Eng., 33, 101113 (2020)
Zhu L, Wu M, Van der Bruggen B, Lei L, Zhu L, Sep. Purif., 242, 116770 (2020)
Kumar R, Isloor AM, Ismail AF, Desalination, 350, 102 (2014)
Esfe MH, Amiri MK, Bahiraei M, J. Taiwan Inst. Chem. E, 103, 7 (2019)
Paduretu CC, Isopescu R, Rau I, Apetroaei MR, Schroder V, Korean J. Chem. Eng., 36(11), 1890 (2019)
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Esfe MH, Kamyab MH, Afrand M, Amiri MK, Pkysica A, 510, 610 (2018)
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Prabhu AA, Mandal B, Dasu VV, Korean J. Chem. Eng., 34(4), 1109 (2017)
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Schmitt F, Banu R, Yeom IT, Do KU, Biochem. Eng. J., 133, 47 (2018)
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Tiwari A, Pal D, Sahu O, Res-Eff Tech., 3, 37 (2017)
Alver A, Kazan Z, Sep. Purif., 230, 115868 (2020)
Choudhury P, Mondal P, Majumdar S, Saha S, Sahoo GC, J. Clean Prod., 203, 511 (2018)
Jun LY, Karri RR, Yon LS, Mubarak N, Bing CH, Mohammad K, Jagadish P, Abdullah E, Environ. Res., 183, 109158 (2020)
Toosi MR, Emami MRS, Hajian S, Environ. Sci. Pollut., 25, 20217 (2018)
Kalaiyarasi M, Ahmad P, Vijayaraghavan P, J. King Saud Univ. Sci., 32, 2134 (2020)
Poorarbabi A, Ghasemi M, Moghaddam MA, Ain Shams Eng. J., In press (2020).
Zhang H, Choi JP, Moon SK. Ngo TH, Addit. Manuf., 33, 101096 (2020)
Ratanasumarn N, Chitprasert P, Int. J. Biol. Macromol., 153, 138 (2020)
Hosseinpour M, Soltani M, Noofeli A, Nathwani J, Fuel, 271, 117618 (2020)
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Juez-Gil M, Erdakov IN, Bustillo A, Pimenov DY, J. Adv. Res., 18, 173 (2019)
Alameer Z, Elaziz MA, Ewees AA, Ye H, Jianhua Z, Resources Policy, 61, 250 (2019)