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Received September 8, 2020
Accepted December 11, 2020
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Decolorization of triarylmethane dyes, malachite green, and crystal violet, by sewage sludge biochar: Isotherm, kinetics, and adsorption mechanism comparison
1Life Green Technology Co. Ltd., 875 Yuseong-daero, Yuseong-gu, Daejeon 34158, Korea 2Department of Chemical and Biological Engineering, Hanbat National University, 125 Dongseo-daero, Yuseong-gu, Daejeon 34158, Korea 3Department of Environmental Engineering, Kyungpook National University, 80 Daehak-ro, Buk-gu, Daegu 41566, Korea 4Department of Electronics Engineering, School of Engineering, Hellenic Mediterranean University, Chania, Crete, Greece
shwoo@hanbat.ac.kr
Korean Journal of Chemical Engineering, March 2021, 38(3), 531-539(9), 10.1007/s11814-020-0727-7
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Abstract
Sewage sludge biochar (SBC) was used as adsorbent to study the adsorption behavior of triarylmethane dyes, malachite green (MG; diaminotriphenylmethane), and crystal violet (CV; triaminotriphenylmethane). SBC exhibited high content (g/kg) of Al (65.8), P (64.6), Ca (57.3), and Fe (44.6). The Langmuir model showed that the affinity of MG for the surface of SBC was 22.6-times that of CV…s (KL=0.0053 l/mg); maximum Langmuir monolayer adsorption capacity of 69.5mg/g for MG and 49.0mg/g for CV. Similar functional groups and adsorption mechanisms like hydrogen bonding, π-π interaction, electrostatic interactions, and ion exchanges governed both MG and CV adsorption onto SBC. Both physisorption and chemisorption were involved in both dyes… adsorption (Redlich-Peterson model: R2> 0.900) Leachability tests showed a dependency of leached metallic ions on the type of dye employed, where ion exchange was dominated by P, Al, Ca, K for MG, and Na, K, Ca for CV. Interestingly, although minimal, the standalone contribution of biochar-free ions on MG and CV decolorization was, respectively, 13% and 7.7% (Fe), 6.7% and 2.3% (K), 2.9% and 0% (Ca), and 0% and 0.8% (Mg), which showed that some adsorption-unrelated mechanism may have also contributed to decolorization of CV and MG.
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Ho YS, McKay G, Can. J. Chem. Eng., 76(4), 822 (1998)
Castellini E, Andreoli R, Malavasi G, Pedone A, Colloids Surf. A: Physicochem. Eng. Asp., 329, 31 (2008)
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Akar E, Altiniskik A, Seki Y, Ecol. Eng., 52, 19 (2013)
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Madhavakrishnan S, Manickavasagam K, Vasanthakumar R, Rasappan K, Mohanraj R, Pattabhi S, E-J. Chem., 6, 1109 (2009)
Guzel F, Saygili H, Saygili GA, Koyuncu F, J. Ind. Eng. Chem., 20(5), 3375 (2014)
Jung H, Sewu DD, Ohemeng-Boahen G, Lee DS, Woo SH, Waste Manage., 91, 33 (2019)
