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Received August 25, 2020
Accepted January 5, 2021
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This is an Open-Access article distributed under the terms of the Creative Commons Attribution Non-Commercial License (http://creativecommons.org/licenses/bync/3.0) which permits
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Ammonia removal by adsorptive clinoptilolite ceramic membrane: Effect of dosage, isothermal behavior and regeneration process
Mohd Ridhwan Adam
Mohd Hafiz Dzarfan Othman†
Siti Hamimah Sheikh Abdul Kadir1
Muthia Elma2
Tonni Agustiono Kurniawan3
Ahmad Fauzi Ismail
Mohd Hafiz Puteh4
Azeman Mustafa
Mukhlis A. Rahman
Juhana Jaafar
Huda Abdullah5
Advanced Membrane Technology Research Centre (AMTEC), School of Chemical and Energy Engineering, Universiti Teknologi Malaysia, 81310 UTM, Skudai, Johor, Malaysia 1Institute of Medical Molecular Biotechnology, Faculty of Medicine, Sungai Buloh Campus, Universiti Teknologi MARA (UiTM), Jalan Hospital, 47000, Sungai Buloh, Selangor, Malaysia 2Chemical Engineering Department, Engineering Faculty, Lambung Mangkurat University, 70714 Banjarbaru, South Kalimantan, Indonesia 3Key Laboratory of the Coastal and Wetland Ecosystems (Xiamen University), Ministry of Education, College of Ecology and the Environment, Xiamen University, Xiamen 361102 Fujian Province, P. R. China 4School of Civil Engineering (FCE), Universiti Teknologi Malaysia, 81310 UTM, Skudai, Johor, Malaysia 5Department of Electrical, Electronic & Systems Engineering, Faculty of Engineering & Built Environment, The National University of Malaysia, Korea
Korean Journal of Chemical Engineering, April 2021, 38(4), 807-815(9), 10.1007/s11814-021-0742-3
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Abstract
This work investigates the effectiveness of ammoniacal nitrogen (NH4 +-N) removal from contaminated water by adsorptive hollow fiber ceramic membrane (HFCM) derived from naturally made clinoptilolite. The technological value of this work is the simple mechanism of the adsorptive HFCM in removing gaseous ammonia in water by combining adsorption and separation. To test the technical feasibility of this proposed technology, clinoptilolite HFCM was fabricated via phase inversion-based extrusion/sintering technique and characterized by SEM and water permeation flux. The produced HFCM corresponds to the desired morphology of the asymmetric structure (dense and void formations) with outstanding adsorption performance of NH4 +-N. The effects of the HFCM…s operational parameters on its removal are examined in terms of membrane dosage and isothermal studies. The adsorption isotherm behavior exhibited that the adsorption process fitted the Freundlich isotherm model with outstanding removal performance even at trace concentration of ammonia. The low amount used by HFCM (4.75⊥10?4m2) resulted in over 96% ammonia removal, indicating a low cost of adsorption process. The regeneration of saturated HFCM suggests an outstanding recovery of the HFCM for its subsequent use for NH4 +-N removal. This study also reveals the potential of adsorptive HFCM as a simple and cost-effective technology for ammonia removal from wastewater.
Keywords
References
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Ilies P, Mavinic DS, Water Res., 35, 2065 (2001)
Yang X, Fraser T, Myat D, Smart S, Zhang J, Diniz da Costa J, Liubinas A, Duke M, Membranes, 4, 40 (2014)
Zhang T, Ding LL, Ren HQ, J. Hazard. Mater., 166(2-3), 911 (2009)
Feng ZM, Sun T, Chem. Eng. J., 281, 295 (2015)
Cheng XW, Zhong Y, Wang J, Guo J, Huang Q, Long YC, Microporous Mesoporous Mater., 83, 233 (2005)
Du Q, Liu SJ, Cao ZH, Wang YQ, Sep. Purif. Technol., 44(3), 229 (2005)
Gunay A, J. Hazard. Mater., 148(3), 708 (2007)
Karadag D, Koc Y, Turan M, Armagan B, J. Hazard. Mater., 136(3), 604 (2006)
Sprynskyy M, Lebedynets M, Terzyk AP, Kowalczyk P, Namiesnik J, Buszewski B, J. Colloid Interface Sci., 284(2), 408 (2005)
Tosun I, Int. J. Environ. Res. Public. Health, 9, 970 (2012)
Adam MR, Salleh NM, Othman MHD, Matsuura T, Ali MH, Puteh MH, Ismail AF, Rahman MA, Jaafar J, J. Environ. Manage., 224, 252 (2018)
Ahmadiannamini P, Eswaranandam S, Wickramasinghe R, Qian XH, J. Membr. Sci., 526, 147 (2017)
Gohari RJ, Lau WJ, Matsuura T, Ismail AF, Sep. Purif. Technol., 118, 64 (2013)
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Adam MR, Othman MHD, Kadir SHSA, Sokri MN, Tai ZS, Iwamoto Y, Tanemura M, Honda S, Membranes, 10, 63 (2020)
Aziz MHA, Othman MHD, Hashim NA, Adam MR, Mustafa A, Appl. Clay Sci., 177, 51 (2019)
Jamil SM, Othman MHD, Mohamed MH, Adam MR, Rahman MA, Jaafar J, Ismail AF, Int. J. Hydrog. Energy, 43(39), 18509 (2018)
Hubadillah SK, Othman MHD, Rahman MA, Ismail AF, Jaafar J, Arab. J. Chem., 13, 2349 (2020)
Adam MR, Salleh NM, Othman MHD, Matsuura T, Ali MH, Puteh MH, Ismail AF, Rahman MA, Jaafar J, J. Environ. Manage., 224, 252 (2018)
Adam MR, et al. Adsorptive natural zeolite ceramic membrane for ammonia removal in wastewater, Editor. 2019, Universiti Teknologi Malaysia: Malaysia (2019).
Verdouw H, Van Echteld CJA, Dekkers EMJ, Water Res., 12, 399 (1978)
Zhou L, Boyd CE, Aquaculture, 450, 187 (2016)
Guillen GR, Pan YJ, Li MH, Hoek EMV, Ind. Eng. Chem. Res., 50(7), 3798 (2011)
Luyten J, Buekenhoudt A, Adriansens W, Cooymans J, Weyten H, Servaes F, Leysen R, Solid State Ion., 135(1-4), 637 (2000)
Adam MR, Othman MHD, Hubadillah SK, Puteh MH, Harun Z, Ismail AF, Int. J. Eng., Trans. B Appl., 31, 1398 (2018)
Moradi M, Karimzadeh R, Moosavi ES, Fuel, 217, 467 (2018)
Amereh M, Haghighi M, Estifaee P, Arab. J. Chem., 11, 81 (2018)
Jamalzadeh Z, Haghighi M, Asgari N, Front. Environ. Sci. Eng., 7, 365 (2013)
Silva MCD, Lira H, Lucena LID, Rosa CD, Freitas OD, Normanda LD, Adv. Mater. Sci. Eng., 2015, 7 (2015)
Opiso E, Sato T, Yoneda T, Int. J. Oil, Gas Coal Technol., 12, 197 (2016)
Angar Y, Djelali NE, Kebbouche-Gana S, Environ. Sci. Pollut., 24, 11078 (2017)
Alshameri A, Yan C, Al-Ani Y, Dawood AS, Ibrahim A, Zhou C, Wang H, J. Taiwan Inst. Chem. Eng., 45, 554 (2014)
Jha VK, Hayashi S, J. Hazard. Mater., 169(1-3), 29 (2009)
Ugrlu M, Karaoglu MH, Microporous Mesoporous Mater., 139, 173 (2011)
Jiang JQ, Cooper C, Ouki S, Chemosphere, 47, 711 (2002)
Taha MR, Geoenvironmental aspects of tropical residual soils, in Tropical residual soils engineering, Taylor & Francis Group, London (2004).
Saltali K, Sari A, Aydin M, J. Hazard. Mater., 141(1), 258 (2007)
Ramirez A, Giraldo S, Garcia-Nunez J, Florez E, Acelas N, J. Water Process. Eng., 26, 131 (2018)
Babel S, Kurniawan TA, J. Hazard. Mater., 97(1-3), 219 (2003)
Elmoubarki R, Mahjoubi FZ, Tounsadi H, Moustadraf J, Abdennouri M, Zouhri A, El Albani A, Barka N, Water Resour. Ind., 9, 16 (2015)
Jorgensen TC, Weatherley LC, Water Res., 37, 1723 (2003)
Yrappa KB, Suresh KBV, Asian J. Chem., 19, 4933 (2007)
Wu H, Zhou W, Pinkerton FE, Meyer MS, Srinivas G, Yildirim T, Udovic TJ, Rush JJ, J. Mater. Chem., 20, 6550 (2010)
Agha MA, Ferrell RE, Hart GF, Ghar MSAE, Abdel-Motelib A, Appl. Clay Sci., 131, 74 (2016)
Uddin MK, Chem. Eng. J., 308, 438 (2017)
Adam MR, Othman MHD, Abu Samah R, Puteh MH, Ismail AF, Mustafa A, Rahman MA, Jaafar J, Sep. Purif. Technol., 213, 114 (2019)
Chia-Hao L, Chin-Hau G, Jia-Jun S, Shing-Yi S, J. Membr. Sci., 471, 285 (2014)
