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Received January 19, 2022
Accepted April 14, 2022
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This is an Open-Access article distributed under the terms of the Creative Commons Attribution Non-Commercial License (http://creativecommons.org/licenses/bync/3.0) which permits
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Synthesis of manganese-iron oxides/activated carbon as a highly effective adsorbent for sulfamerazine pollutant removal
1Center for Environment and Water Resource, College of Chemistry and Chemical Engineering, Central South University, Changsha 410083, P. R. China 2Key Laboratory of Hunan Province for Water Environment and Agriculture Product Safety, Changsha 410083, P. R. China
Korean Journal of Chemical Engineering, November 2022, 39(11), 3083-3091(9), 10.1007/s11814-022-1147-7
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Abstract
Considering the frequent detection in environment and the potential threat to human health and ecoenvironment, achieving removal of sulfamerazine (SMZ) from the aquatic environment is of great significance. In this study, the magnetically separable manganese-iron oxides/activated carbon (Mn-Fe3O4/AC) was synthesized by simple co-precipitation method and was used to remove SMZ from solution. Doping manganese oxide could change the specific surface areas of the prepared materials, thus providing more active sites for adsorption and improving the adsorption capacity of Mn-Fe3O4/AC for SMZ (maximum adsorption capacity 146mg g-1). The kinetic and thermodynamic study showed that the adsorption of SMZ on Mn-Fe3O4/AC was endothermic and spontaneous, and followed the pseudo-second-order kinetics model and Langmuir model. Efficient removal of SMZ was attributed to varieties of noncovalent interactions between it and Mn-Fe3O4/AC, including electrostatic interactions, hydrogen bonds and π-π electron donor-acceptor interactions. In addition, SMZ could be degraded by oxidation via redox reactions. After six cycles of use, Mn-Fe3O4/AC still had good adsorption capability.
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References
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Wang J, Tao H, Lu T, Wu Y, J. Colloid Interface Sci., 584, 114 (2021)
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Liu X, Gao M, Qiu W, Khan ZH, Liu N, Lin L, Song Z, Environ. Sci. Pollut. Res., 26, 17373 (2019)
