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Received October 20, 2021
Accepted January 15, 2022
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This is an Open-Access article distributed under the terms of the Creative Commons Attribution Non-Commercial License (http://creativecommons.org/licenses/bync/3.0) which permits
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Metal organic frameworks template-directed fabrication of rod-like hollow BiOClxBr1-xwith adjustable band gap for excellent photocatalytic activity under visible light
Ze Luo1
Jinlong Li1 2†
Guozhe Sui1 2†
Yan Zhuang1 3
Dongxuan Guo1 2
Rongping Xu1 3
Shuang Liang1 3
Hong Yao1 3
Chao Wang1 3
Shijie Chen1 2
1College of Chemistry and Chemical Engineering, Qiqihar University, Qiqihar 161006, P. R. China 2Heilongjiang Provincial Key Laboratory of Catalytic Synthesis for Fine Chemicals, Qiqihar University, Qiqihar 161006, P. R. China 3, China
jinlong141@163.com
Korean Journal of Chemical Engineering, August 2022, 39(8), 2127-2137(11), 10.1007/s11814-022-1070-y
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Abstract
Developing an efficient, environmentally friendly, and pollution-free catalyst with excellent visible light catalytic activity is a promising strategy for dye wastewater treatment. Herein, the rod-like hollow BiOClxBr1-x (x=1, 0.75, 0.5, 0.25, 0), with an adjustable band gap, was successfully prepared using Bi-based metal-organic framework as template. The corresponding hollow assembly and introduction of Br- imparted valuable structural advantages and intrinsic characteristics for improved photocatalytic activity. Significantly, the degradation efficiency of BiOCl0.5Br0.5 for the Rhodamine B (RhB) solution reached 92% under visible light illumination for 90 min, which is considerably higher than that of CAU-17-derived Bi2O3 and BiOCl. Overall, these findings shed fundamental insight on constructing novel photocatalysts with excellent visible light driven photocatalytic activity and offered a new method for treating dye wastewater.
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