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Received February 1, 2022
Accepted May 11, 2022
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This is an Open-Access article distributed under the terms of the Creative Commons Attribution Non-Commercial License (http://creativecommons.org/licenses/bync/3.0) which permits
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A short review on hydrophobic pervaporative inorganic membranes for ethanol/water separation applications
1Decommissioning Technology Research Division, Korea Atomic Energy Research Institute, 989-111 Daedeok-daero, Yuseong-gu, Daejeon 34057, Korea 2Nuclear Research Institute for Future Technology and Policy, Seoul National University, 1 Gwanak-ro, Gwanak-gu, Seoul 08826, Korea
Korean Journal of Chemical Engineering, September 2022, 39(9), 2263-2274(12), 10.1007/s11814-022-1173-5
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Abstract
Inorganic based membranes are promising candidates for a variety of applications, including adsorption and separation due to their large surface area, high pore volume, tunable structure, and strong resistance against aggressive operation conditions, such as high temperature and pressure. Many research groups have investigated zeolite, micro- or mesoporous silica, and hybrid materials (organic and inorganic materials) as advanced membrane configurations in liquid separation applications. Especially, hydrophobic inorganic membranes have potential to separate ethanol from aqueous solution via pervaporation, ultimately producing ethanol, but several important challenges such as reliable synthesis, fabrication, or functionalization are yet to be solved. More specifically, a novel, high throughput process for the fabrication of continuous and defect-free hydrophobic inorganic membranes is required. Then, functionalization of pore structures of the membrane, if necessary, is desirable in order to tailor even more advanced hydrophobic properties for ethanol. Finally, the separation characteristics and performance of inorganic membranes must be further investigated to implement in the industry. Herein, the synthesis and normalized separation performance of diverse hydrophobic inorganic membranes with respect to selective layer material basis, such as zeolite, functionalized mesoporous silica, and mixed matrix, are comprehensively reviewed and the future direction is presented with a focus on ethanol recovery.
Keywords
References
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Mohammadi T, Pak A, Microporous Mesoporous Mater., 56, 81 (2002)
Wong WC, Au LTY, Ariso CT, Yeung KL, J. Membr. Sci., 191, 143 (2001)
Tuan VA, Falconer JL, Noble RD, Ind. Eng. Chem. Res., 38, 3635 (1999)
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Lin X, Kita H, Okamoto KI, Ind. Eng. Chem. Res., 40, 4069 (2001)
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Wei Q, Ding YL, Nie ZR, Liu XG, Li QY, J. Membr. Sci., 466, 114 (2014)
Koyano KA, Tatsumi T, Tanaka Y, Nakata S, J. Phys. Chem. B, 101, 9436 (1997)
Kujawski W, Roszak R, Sep. Sci. Technol., 37, 3559 (2002)
Kujawski W, Kujawa J, Wierzbowska E, Cerneaux S, Bryjak M, Kujawski J, J. Membr. Sci., 499, 442 (2016)
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Vinh-Thang H, Kaliaguine S, Chem. Rev., 113, 4980 (2013)
Ren H, Jin J, Hu J, Liu H, Ind. Eng. Chem. Res., 51, 10156 (2012)
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Amrei SS, Asghari M, Esfahanian M, Zahraei Z, J. Chem. Technol. Biotechnol., 95, 1604 (2020)
Çalhan A, Deniz S, Romero J, Hasanoğlu A, Korean J. Chem. Eng., 36, 1489 (2019)
Mizsey P, Selim A, Toth AJ, Fozer D, Süvegh K, ACS Omega, 5, 32373 (2020)
Kulkarni AS, Sajjan AM, Ashwini M, Banapurmath NR, Ayachit NH, Shirnalli GG, RSC Adv., 10, 22645 (2020)
Grzybek P, Jakubski L, Borys P, Kołodziej S, Ślusarczyk C, Turczyn R, Dudek G, Sep. Purif. Technol., 281, 119897 (2022)
Dudek G, Turczyn R, Djurado D, Materials, 13, 4152 (2020)
Pan F, Cao C, Liu G, Jiang Z, Chem. Eng. Sci. X, 11, 100102 (2021)
Castro-Muñoz R, Boczkaj G, Molecules, 26, 1242 (2021)
Hasegawa Y, Abe C, Ikeda A, Membranes, 11, 229 (2021)
Li L, Lu Y, Li L, Yang J, Fu W, Luo Y, Lu J, Zhang Y, Zhou L, J. Membr. Sci., 638, 119701 (2021)
