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Received November 16, 2021
Accepted May 14, 2022
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This is an Open-Access article distributed under the terms of the Creative Commons Attribution Non-Commercial License (http://creativecommons.org/licenses/bync/3.0) which permits
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Composites of poly(vinyl pyrrolidone) and polarized Ag nanoparticles for CO2 separation
1Department of Chemistry, Sangmyung University, Seoul 03016, Korea 2Department of Chemistry and Energy Engineering, Sangmyung University, Seoul 03016, Korea
swkang@smu.ac.kr
Korean Journal of Chemical Engineering, September 2022, 39(9), 2542-2547(6), 10.1007/s11814-022-1179-z
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Abstract
A poly(vinyl pyrrolidone) (PVP)/Ag nanoparticles (AgNPs)/7,7,8,8-Tetracyanoquinodimethane (TCNQ)/ dioctyl phthalate (DOP) composite membrane using positively charged silver nanoparticles was prepared for CO2 separation. Positively polarized silver nanoparticles were generated by TCNQ, known as an electron acceptor for CO2 carrier. In the separation of CO2 and N2, the composite membrane consisting of PVP/AgNPs/TCNQ/DOP showed that only polar CO2 could be selectively separated by a reversible reaction with the positively polarized silver nanoparticles. Furthermore, the addition of DOP as a plasticizer enhanced gas permeance through the glassy PVP, and the CO2/N2 selectivity performance reached 103.8. The PVP/AgNPs/TCNQ/DOP composite membranes were characterized by FTIR spectroscopy, X-ray photoelectron spectroscopy, thermogravimetric analysis, and scanning electron microscopy.
Keywords
References
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