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Received March 30, 2022
Accepted August 2, 2022
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This is an Open-Access article distributed under the terms of the Creative Commons Attribution Non-Commercial License (http://creativecommons.org/licenses/bync/3.0) which permits
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Kinetic and thermodynamic evaluation of pyrolysis of jeans waste via coats-redfern method
Rumaisa Tariq1
Abrar Inayat2
Muhammad Shahbaz3
Hassan Zeb4†
Chaouki Ghenai2
Tareq Al-Ansari3
Jaehoon Kim5 6†
1School of Engineering, Monash University Malaysia, 47500 Bandar Sunway, Malaysia 2Department of Sustainable and Renewable Energy Engineering, University of Sharjah, 27272, Sharjah, United Arab Emirates 3Division of Sustainable Development, College of Science and Engineering, Hamad Bin Khalifa University (HBKU), Qatar Foundation, 5825 Doha, Qatar 4Institute of Energy and Environmental Engineering, University of the Punjab, Q&A Campus, Lahore, Pakistan 5SKKU Advanced Institute of Nanotechnology (SAINT), Sungkyunkwan University, 2066 Seobu-ro, Jangan-gu, Suwon, Gyeong Gi-do 16419, Korea 6School of Mechanical Engineering, Sungkyunkwan University, 2066 Seobu-ro, Jangan-gu, Suwon, Gyeong Gi-do 16419, Korea
hassanzeb.ieee@pu.edu.pk
Korean Journal of Chemical Engineering, January 2023, 40(1), 155-161(7), 10.1007/s11814-022-1248-3
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Abstract
Used textiles, such as jeans wastes, exhibit a high potential for generating renewable and sustainable energy. However, limited research has been devoted toward investigating the kinetic and thermodynamic parameters of textile wastes during pyrolysis and applying these wastes as feedstock for fuels such as biogas. Therefore, this study investigated the kinetic and thermodynamic aspects of the thermal decomposition of jeans waste to evaluate its potential for sustainable energy production. Jeans waste was heat treated at 50-850 ℃ under different heating rates of 10-40 ℃ min-1. Active pyrolysis for the decomposition of jeans waste occurred at temperatures ranging from 250 to 550 ℃. Specific Coats-Redfern-type reaction mechanisms were applied to determine the kinetic and thermodynamic variables in the active temperature zone. The thermodynamic parameters (ΔH and ΔG) and activation energies increased when the heating rate was increased from 10 to 30 ℃ min-1. When the heating rate was further increased to 40 ℃ min-1, ΔH, ΔG, and the activation energies decreased. For heating rates of 10, 20, 30, and 40 ℃ min-1, the pre-exponential factors varied in the ranges of 7.4×103 to 1.4×104, 1.8×104 to 5.1×1010, 2.8×104 to 5.3×1010, and 3.6×104 to 3.1×1010 min-1, respectively. In each reaction mechanism model, the entropy changed negatively for all the heating rates examined in this study. This work and its results could serve as a guide for implementing such pyrolysis processes for textile wastes at a practical scale for bioenergy applications.
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Kim YM, Jae J, Kim BS, Hong Y, Jung SC, Park YK, Energy Conv. Manag., 149, 966 (2017)
Valizadeh S, Lam SS, Ko CH, Lee SH, Farooq A, Yu YJ, Jeon JK, Jung SC, Rhee GH, Park YK, Bioresour. Technol., 320, 124313 (2021)
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Yousef S, Eimontas J, Striūgas N, Tatariants M, Abdelnaby MA, Tuckute S, Kliucininkas L, Energy Conv. Manag., 196, 688 (2019)
Naqvi SR, Tariq R, Hameed Z, Ali I, Naqvi M, Chen WH, Ceylan S, Rashid H, Ahmad J, Taqvi SA, Renew. Energy, 131, 854 (2019)
Mishra G, Kumar J, Bhaskar T, Bioresour. Technol., 182, 282 (2015)
Naqvi SR, Hameed Z, Tariq R, Taqvi SA, Ali I, Niazi MBK, Noor T, Hussain A, Iqbal N, Shahbaz M, Waste Manage., 85, 131 (2019)
Motghare KA, Rathod AP, Wasewar KL, Labhsetwar NK, Waste Manage., 47, 40 (2016)
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Szabó T, Berkesi O, Forgó P, Josepovits K, Sanakis Y, Petridis D, Dékány I, Chem. Mater., 18, 2740 (2006)
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Turmanova SC, Genieva SD, Dimitrova AS, Vlaev LT, Express Polym. Lett., 2, 133 (2008)
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