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Received April 19, 2022
Accepted August 17, 2022
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This is an Open-Access article distributed under the terms of the Creative Commons Attribution Non-Commercial License (http://creativecommons.org/licenses/bync/3.0) which permits
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Downstream process development of biobutanol using deep eutectic solvent
Dept. of Chem. & Energy Eng., Kyungnam Coll. of Info. & Tech., Busan 47011, Korea 1Dept. of Industrial Chemistry, Pukyong National University, Busan 48547, Korea
Korean Journal of Chemical Engineering, January 2023, 40(1), 205-214(10), 10.1007/s11814-022-1265-2
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Abstract
Biobutanol is produced from lignocellulose fermentation. Owing to the abundance of this feedstock and the similarities between the properties of biobutanol and gasoline, biobutanol represents a promising alternative to current crude-oil-based automotive fuel. Environmentally friendly recovery of biobutanol from the fermentation products is essential for achieving carbon-neutral production. Because extraction substantially lowers the energy demand for distillation, an eco-friendly deep eutectic solvent (DES) was applied for biobutanol extraction here, and the non-random two-liquid (NRTL) parameters that were compatible with the process design program were derived using experimental measurements and molecular simulations. For the liquid-liquid equilibrium (LLE) parameter estimation, a non-iterative procedure was introduced with a suitable arrangement of binary parameters for the DES. Compared to previous studies, the process design results indicate a marked reduction in energy consumption for the near-complete recovery of high-purity biobutanol, requiring a comparable investment.
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References
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