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Received August 18, 2022
Revised November 10, 2022
Accepted January 31, 2023
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Recent progress in the preparation, characterization, and applications of modified halloysite nanotubes as adsorbents for wastewater treatment
Zaharaddeen Nasiru Garba1†
Abdurrashid Haruna2
Abdulkadir Tanimu3
Binta Zakari Bello4
Zakariyya Uba Zango5†
1Department of Chemistry, Ahmadu Bello University, P.M.B. 1044, Zaria, Nigeria 2Department of Fundamental and Applied Sciences, Universiti Teknologi PETRONAS, 32610 Seri Iskandar, Perak Darul Ridzuan, Malaysia 3Centre for Refining and Advanced Chemicals, King Fahd University of Petroleum and Minerals, Dhahran 31261, Saudi Arabia 4Department of Chemical Engineering, Ahmadu Bello University Zaria, Nigeria 5Institute of Semi-Arid Zone Studies, Al-Qalam University Katsina, P.M.B. 2137, Katsina, Nigeri
zngarba@abu.edu.ng, dinigetso2000@gmail.com
Korean Journal of Chemical Engineering, June 2023, 40(6), 1247-1267(21), 10.1007/s11814-023-1440-0
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Abstract
The application of halloysite nanotubes (HNTs) in water purification is attracting extensive attention
because they are inexpensive raw materials with a hollow nanotubular structure in the sub-micrometer range, a large
specific surface area, pore volume, pore size, and adequate hydroxyl groups on their surface, thus enhancing their ability to be modified. These modified halloysite nanotubes (m-HNTs) have been widely used for a variety of applications,
including chemocatalysis, biocatalysis, antibacterial action, drug delivery, gas separation, and adsorbents for wastewater
treatment. They were reported to have been produced using a variety of synthetic processes which include self-assembly/vacuum filtering, extraction, solution casting, dehydration condensation, thermal polycondensation, chemical vapor
deposition, and hydrothermal carbonization. In this review, we focus on the compilation of the most recent developments in the manufacture of m-HNTs, their characterization and possible uses in wastewater treatment. Finally, we
present our personal views on the opportunities and challenges of future researches involving m-HNTs, hoping to
inspire more researchers into participating in this fascinating area.
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