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Guidelines for the Design of Solid CO 2 Adsorbents for Mobile Carbon Capture in Heavy-Duty Vehicles: A Review

Department of Energy Systems Research , Ajou University , 206 Worldcup-ro Yeongtong-gu , Suwon 16499 , Korea 1Plant Engineering Center, Institute for Advanced Engineering , Yongin 17180 , Korea 2Plant Engineering Center, Institute for Advanced Engineering , Yongin 17180 , Korea
Korean Journal of Chemical Engineering, January 2024, 41(1), 25-42(18), https://doi.org/10.1007/s11814-024-00053-0

Abstract

The transportation sector is the largest contributor to carbon dioxide (CO 2 ) emissions, largely due to heavy-duty vehicles

(HDVs) that inevitably rely on internal combustion engines. Electrifi cation is a promising technology for decarbonizing

light-duty vehicles but it is diffi cult to apply to HDVs with long driving ranges and signifi cant weights. One possible solution

is a mobile carbon capture (MCC) system that adapts onboard CO 2 capture and storage to the HDV. Although conceptual

designs have been presented for MCC systems that use adsorbents and temperature-swing adsorption (TSA), the development

of the adsorbent-based MCC remains in its infancy. Since adsorbents play a critical role in determining the overall weight,

volume, and energy consumption of the MCC, the development of a high performance adsorbent is a key factor in the successful

MCC design. In this review, we aim to provide guidelines for the design of CO 2 adsorbents for MCC in HDVs. First,

we briefl y introduce the adsorbent selection criteria for TSA in MCC, including the CO 2 working capacity, purity, stability,

and regeneration energy. Then, we summarize recent progress in the development of adsorbents tested under MCC-relevant

conditions. Finally, the current challenges and future prospects of MCC are discussed.

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