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Received October 7, 2020
Accepted December 13, 2020
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A short review on dissolved lithium polysulfide catholytes for advanced lithium-sulfur batteries
Department of Engineering Chemistry, Chungbuk National University, Chungbuk 28644, Korea 1Department of Chemical Engineering, Gyeongsang National University, 501 Jinju-daero 52828, Korea
jscho@cbnu.ac.kr
Korean Journal of Chemical Engineering, March 2021, 38(3), 461-474(14), 10.1007/s11814-020-0729-5
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Abstract
Lithium-sulfur battery (LSB) technology has drawn enormous attention during the last decade. Benefitting from the high theoretical specific discharge capacity (1,675mAh g-1) and energy density (2,600Wh kg-1), LSBs have proved to be a suitable candidate for electric vehicles and large-scale power grid electrical energy storage systems. However, the commercialization of LSB is hindered by various barriers, which include the high insulating nature of sulfur and its discharge products, severe polysulfide shuttling phenomenon, extreme volume expansion during charging/discharging, and poor stability of Li metal anodes. Additionally, LSB technology faces considerable battery design challenges, which allows high sulfur content and/or sulfur-loading while simultaneously maintaining a low electrolyte/ sulfur ratio. Therefore, in this review, we highlight recent effective strategies that lead to more practical and commercial LSBs. We restrict ourselves to various cathode architectures designed specifically to absorb dissolved polysulfide catholyte. The integration of dissolved lithium polysulfide catholyte with specially designed cathode substrates efficiently allows ultra-high sulfur loading and/or sulfur-content with low electrolyte/sulfur ratio while still exhibiting reasonable electrochemical performance and cycling stability. The effect of concentration variation of dissolved lithium polysulfide catholyte on the cell performance is also discussed in detail. Therefore, the present review encapsulates feasible strategies with practical parameters to address the problems associated with LSBs.
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References
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